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Record W4249153173 · doi:10.1149/ma2016-01/33/1623

Electrochemical Studies of L-Cysteine

2016· article· en· W4249153173 on OpenAlexaboutno aff
Graham T. Cheek, Matthew A. Worosz

Bibliographic record

VenueECS Meeting Abstracts · 2016
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsnot available
Fundersnot available
KeywordsChemistryCystineElectrochemistryInorganic chemistryPlatinumPotentiostatCysteineElectrolysisGlassy carbonCyclic voltammetryAqueous solutionElectrodeRedoxVoltammetryOrganic chemistryElectrolytePhysical chemistryCatalysis

Abstract

fetched live from OpenAlex

Introduction L-Cysteine is an important amino acid because of its role in various biochemical pathways (1). Considering that L-cysteine is one of the few amino acids with significant redox characteristics, it was considered worthwhile to investigate its electrochemical behavior in various media and electrode surfaces. Experimental L-Cysteine was obtained from Sigma-Aldrich. Electrochemical experiments were carried out using a Gamry Interface 1000 potentiostat and Gamry Framework software. Potentials are referenced against a Ag/AgCl reference electrode. Platinum and glassy carbon electrodes were obtained from BASi. Results and Discussion At a platinum electrode, L-cysteine in aqueous 0.10 M KNO 3 produced a cyclic voltammogram with two merged oxidation processes (Figure 1), which were much more clearly resolved using differential pulse voltammetry. Preparative electrolysis at the potential of the first oxidation process (+0.80 V) resulted in the precipitation of cystine, which is the coupling product formed as a result of one-electron L-cysteine oxidation. The current for the reduction peak at -0.60 V (dotted line in Figure 1) increased during the electrolysis, suggesting that this reduction process is related to cystine formation. Similar results, including cystine formation, were also obtained in aqueous phosphate buffer at pH 7. It is likely that the platinum oxide layer on the electrode surface plays a role in L-cysteine oxidation under these conditions (2). The results of additional studies of L-cysteine oxidation in other media, particularly dimethylsulfoxide (DMSO), are also planned for presentation. References C. K. Mathews, K. E. Van Holde, D. R. Appling, and S. J. Anthony-Cahill, Biochemistry, 4 th Edition , Pearson Canada, Toronto, 2013. J. Koryta and J. Pradac, J. Electroanal. Chem. , 17 , 185-189 (1968). Figure 1. Cyclic voltammogram of 10 mM L-cysteine at platinum in aqueous 0.10 M KNO 3 . 100 mV/s. First sweep (solid line), second sweep (dotted line). Figure 1

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.184

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.035
GPT teacher head0.297
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2016
Admission routes1
Has abstractyes

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