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Record W4249309218 · doi:10.1055/s-0029-1219042

Triphenylcarbenium Tetrafluoroborate

2010· article· en· W4249309218 on OpenAlexaff
Huan Liang

Bibliographic record

VenueSynlett · 2010
Typearticle
Languageen
FieldChemistry
TopicChemical Synthesis and Reactions
Canadian institutionsUniversity of British Columbia
Fundersnot available
KeywordsChemistryAcetic anhydrideDehydrogenationOrganic chemistryDichloromethaneCationic polymerizationTetrahydrofuranCatalysisSilylationTetrafluoroborateLewis acids and basesKetoneAnhydrousAcetic acidCarbocationPolymer chemistryIonic liquidSolvent

Abstract

fetched live from OpenAlex

All articles of this category Introduction Triphenylcarbenium tetrafluoroborate, also called trityl fluoroborate, is widely applied in organic reactions, [ ¹ ] such as dehydrogenation, [ ² ] deprotection of ketone acetals, [ ³ ] alkyl ethers, [ 4 ] oxidation of silyl enol ethers, [ 5 ] preparation of cationic organometallics [ 6 ] or organic complexes, [ 7 ] as a polymerization catalyst [ 8 ] and as a Lewis acid catalyst. [ 9 ] Trityl fluoroborate is a yellow solid (mp 200 ˚C dec.), which is soluble in most organic solvents, e.g., dichloromethane, tetrahydrofuran, and reacts with nucleophilic solvents, e.g., water. Several preparation methods were described in the literature as early as the 1940s. Dauben et al. used triphenylcarbinol and 48% fluoroboric acid, while removing water from the reaction mixture by adding acetic anhydride. [ ¹0a ] In 1972, Olah et al. developed a more convenient and economical route using trityl chloride and anhydrous tetrafluoroboric acid dimethyl etherate in dry benzene. [ ¹0b ] Scheme 1 Improved multi-gram preparation of trityl fluoroborate

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.035

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0100.005

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.208
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2010
Admission routes1
Has abstractyes

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