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Record W4283071038 · doi:10.1002/adom.202200862

Solution‐Based Integration of Vertically Stacked Organic Photodetectors Toward Easy‐To‐Fabricate Filterless Multi‐Color Light Sensors

2022· article· en· W4283071038 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueAdvanced Optical Materials · 2022
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsSimon Fraser University
FundersNational Natural Science Foundation of China
KeywordsPhotodetectorMaterials scienceOptoelectronicsPhotodetectionPhotodiodePhotocurrentPhotonicsFabricationComputer science

Abstract

fetched live from OpenAlex

Abstract Solution‐processed, color‐selective organic photodetectors are uniquely positioned to deliver high‐performance, low‐cost, multicolor light sensors/imagers beyond the limitations of conventional, color‐filter‐based technologies. To realize such potential, however, a prominent challenge has been the solution‐based, monolithic integration of vertically stacked organic photodetectors, which would enable multicolor sensing with optimum light collection while benefiting from the scalability, cost, and sustainability edges of solution‐based manufacturing. To tackle this challenge, this paper demonstrates, for the first time, the monolithic integration of vertically stacked solution‐processed organic photodetectors for independent, multicolor light sensing within the same pixel area. The solvent orthogonality challenge is tackled by selecting polymer‐based photoactive layers and an insulating polymeric spacer—for independent biasing and photocurrent readout—with compatible processing conditions. Based on the suitable characteristics of blue‐ and green‐sensitive standalone devices, the vertically stacked, monolithic device architecture is optimized by also incorporating semitransparent electrodes for photons to reach deep into the stack. The resultant device architecture enables efficient blue‐ and green‐selective photodetection with state‐of‐the‐art linearity, alongside speed of response adequate for real‐world applications. Based on its solution‐processability and modularity, this approach paves the way for the facile, solution‐based fabrication of organic imagers covering multiple spectral regions with high sensitivity and resolution.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.030
GPT teacher head0.282
Teacher spread0.252 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it