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Effect of Naphthenic Acid and Metal Ions on Emulsification of Heavy Oil

2022· article· en· W4283369692 on OpenAlexaboutno aff
Huajian Zhu, Qiang Wang, Yishu Yan, Yinxiang Xu, Shenglan Liu, Shengfei Zhang, Junbo Xu, Chao Yang

Bibliographic record

VenueEnergy & Fuels · 2022
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsnot available
FundersChina Postdoctoral Science FoundationMinistry of Science and Technology of the People's Republic of ChinaNational Natural Science Foundation of China
KeywordsEmulsionAsphalteneNaphthenic acidMetal ions in aqueous solutionChemistryMetalViscosityChemical engineeringExtraction (chemistry)MoleculePhase (matter)ChromatographyMaterials scienceOrganic chemistry

Abstract

fetched live from OpenAlex

The emulsification of heavy oil is universal in various stages of heavy oil extraction, processing, and transportation. In this study, molecular dynamics simulations were employed to reveal the emulsification of heavy oil from different regions. When the water mass fraction is low, metal ions in the Karamay emulsion exist at the oil–water interface and interact with naphthenic acid (NA), which results in strong emulsion stability. The dominant interactions between resin and water molecules cause weak emulsion stability for Liaohe and Canada heavy oils. On the basis of the thermodynamic analysis, we found that the interaction between the metal ion and NA in the Karamay emulsion is much stronger than the interaction between the asphaltene/resin molecules and water molecules in Liaohe and Canada emulsions, which is the main reason for stronger emulsion stability in the Karamay region. As the water concentration increases, the emulsion stability of Karamay heavy oil will have a significant change as a result of the lower metal ion concentration. The water-phase structures and emulsion viscosity were investigated, and the water aggregations present spherical, worm-like, stick, net, and honeycomb structures with the increase of the water concentration. The breakup of the emulsion structure leads to a sudden decrease in the viscosity of the Karamay heavy oil.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.234
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2022
Admission routes1
Has abstractyes

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