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Record W4283375578 · doi:10.5194/acp-22-8221-2022

Transport of substantial stratospheric ozone to the surface by a dying typhoon and shallow convection

2022· article· en· W4283375578 on OpenAlexaff
Zhixiong Chen, Jane Liu, Xiushu Qie, Xugeng Cheng, Yukun Shen, Mengmiao Yang, Rubin Jiang, Xiangke Liu

Bibliographic record

VenueAtmospheric chemistry and physics · 2022
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsUniversity of Toronto
FundersFujian Normal UniversityNational Natural Science Foundation of China
KeywordsRadiosondeOzoneAtmospheric sciencesTroposphereEnvironmental scienceOzone layerClimatologyMesoscale meteorologyStratosphereMeteorologyGeologyGeography

Abstract

fetched live from OpenAlex

Abstract. Stratospheric ozone transported to the troposphere is estimated to account for 5 %–15 % of the tropospheric ozone sources. However, the chances of intruded stratospheric ozone reaching the surface are low. Here, we report an event of a strong surface ozone surge of stratospheric origin in the North China Plain (NCP, 34–40∘ N, 114–121∘ E) during the night of 31 July 2021. The hourly measurements reveal surface ozone concentrations of up to 80–90 ppbv at several cities over the NCP from 23:00 LST (Local Standard time, = UTC +8 h) on 31 July to 06:00 LST on 1 August 2021. The ozone enhancement was 40–50 ppbv higher than the corresponding monthly mean. A high-frequency surface measurement indicates that this ozone surge occurred abruptly, with an increase reaching 40–50 ppbv within 10 min. A concurrent decline in surface carbon monoxide (CO) concentrations suggests that this surface ozone surge might have resulted from the downward transport of a stratospheric ozone-rich and CO-poor air mass. This is further confirmed by the vertical evolutions of humidity and ozone profiles based on radiosonde and satellite data respectively. Such an event of stratospheric impact on surface ozone is rarely documented in view of its magnitude, coverage, and duration. We find that this surface ozone surge was induced by a combined effect of dying Typhoon In-fa and shallow local mesoscale convective systems (MCSs) that facilitated transport of stratospheric ozone to the surface. This finding is based on analysis of meteorological reanalysis and radiosonde data, combined with high-resolution Weather Research and Forecasting (WRF) simulation and backward trajectory analysis using the FLEXible PARTicle (FLEXPART) particle dispersion model. Although Typhoon In-fa on the synoptic scale was at its dissipation stage when it passed through the NCP, it could still bring down a stratospheric dry and ozone-rich air mass. As a result, the stratospheric air mass descended to the middle-to-low troposphere over the NCP before the MCSs formed. With the pre-existing stratospheric air mass, the convective downdrafts of the MCSs facilitated the final descent of stratospheric air mass to the surface. Significant surface ozone enhancement occurred in the convective downdraft regions during the development and propagation of the MCSs. This study underscores the substantial roles of weak convection in transporting stratospheric ozone to the lower troposphere and even to the surface, which has important implications for air quality and climate change.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.395
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.187
Teacher spread0.180 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2022
Admission routes1
Has abstractyes

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