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Performance Metrics to Compare Various CO2 Reduction Processes

2022· article· en· W4283752136 on OpenAlexaff
Katherine Lochhead, Guenevere O’Hara, Dongfang Yang

Bibliographic record

VenueCurrent Alternative Energy · 2022
Typearticle
Languageen
FieldEnergy
TopicCO2 Reduction Techniques and Catalysts
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsMetric (unit)Reduction (mathematics)Computer scienceProcess engineeringWork (physics)Performance metricPhotocatalysisEnvironmental economicsEnvironmental scienceBusinessMathematicsOperations managementCatalysisMechanical engineeringEngineeringChemistry

Abstract

fetched live from OpenAlex

Abstract: In response to the increasing concentration of anthropogenic CO2 in the atmosphere, large research efforts have been placed on the development of suitable carbon capture and utilization technology. The transformation of CO2 into value-added chemicals is one of the most promising routes for carbon utilization and can be accomplished by thermocatalytic, photocatalytic, electrochemical, and photoelectrochemical methods. The advancement of this technology towards a commercial solution requires a synergistic approach, wherein members of the research community are continuously evaluating the comparative performance of each method and adapting their research directions in response. As a result, the establishment of a universal metric for reporting the performance of thermocatalytic, photocatalytic, electrochemical, and photoelectrochemical CO2 reduction processes is critical. This work summarizes the advantages and disadvantages associated with each CO2 reduction method and identifies their most frequently used performance metrics. Subsequently, a new performance metric, which applies to all CO2 reduction technologies, is introduced and defined as the moles formed of the desired product per hour per accessible surface area of catalyst. Although limitations with ease of measurement exist, this work aims to demonstrate how the adoption of a universal performance metric could help to unite the research community towards a common goal and improve its efficiency in finding a solution to the global energy crisis.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.915
Threshold uncertainty score0.859

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.036
GPT teacher head0.295
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2022
Admission routes1
Has abstractyes

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