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Record W4283837355 · doi:10.1021/acs.nanolett.2c00944

Vibronic Exciton–Phonon States in Stack-Engineered van der Waals Heterojunction Photodiodes

2022· article· en· W4283837355 on OpenAlexaff
Fatemeh Barati, Trevor Arp, Shanshan Su, Roger K. Lake, Vivek Aji, Rienk van Grondelle, Mark S. Rudner, Justin C. W. Song, Nathaniel M. Gabor

Bibliographic record

VenueNano Letters · 2022
Typearticle
Languageen
FieldMaterials Science
Topic2D Materials and Applications
Canadian institutionsCanadian Institute for Advanced Research
FundersH2020 European Research CouncilArmy Research OfficeDivision of Materials ResearchDivision of Emerging Frontiers in Research and InnovationDivision of PhysicsNational Aeronautics and Space AdministrationCopenhagen Graduate School for Nanoscience and NanotechnologyU.S. NavyNational Science FoundationUniversity of WashingtonVrije Universiteit AmsterdamNanyang Technological UniversityMinistry of Education, IndiaKoninklijke Nederlandse Akademie van WetenschappenEuropean CommissionMinistry of Education - SingaporeAir Force Office of Scientific ResearchDivision of Mathematical SciencesVillum Fonden
KeywordsPhotocurrentExcitonPhotodiodeHeterojunctionOptoelectronicsvan der Waals forceStack (abstract data type)Materials scienceStackingVibronic couplingBiophotonicsChemistryMolecular physicsCondensed matter physicsPhotonicsPhysicsMolecule

Abstract

fetched live from OpenAlex

heterojunction photodiodes. To do so, we introduce the photocurrent spectroscopy of a stack-engineered photodiode as a sensitive technique for probing interlayer excitons, enabling access to vibronic states typically found only in molecule-like systems. The vibronic states in our stack are manifest as a palisade of pronounced periodic sidebands in the photocurrent spectrum in frequency windows close to the interlayer exciton resonances and can be shifted "on demand" through the application of a perpendicular electric field via a source-drain bias voltage. The observation of multiple well-resolved sidebands as well as their ability to be shifted by applied voltages vividly demonstrates the emergence of interlayer exciton vibronic structure in a stack-engineered optoelectronic device.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.042
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.218
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2022
Admission routes1
Has abstractyes

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