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Record W4285005400 · doi:10.3390/polym14142802

Crystallinity and Gas Permeability of Poly (Lactic Acid)/Starch Nanocrystal Nanocomposite

2022· article· en· W4285005400 on OpenAlex
Somayeh Sharafi Zamir, Babak Fathi, Abdellah Ajji, Mathieu Robert, Saïd Elkoun

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenuePolymers · 2022
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsPolytechnique MontréalMcGill UniversityUniversité de Sherbrooke
FundersFonds de recherche du Québec – Nature et technologies
KeywordsCrystallinityNanocompositeNanocrystalLactic acidStarchChemical engineeringMaterials sciencePermeability (electromagnetism)ChemistryPolymer chemistryComposite materialOrganic chemistryNanotechnologyBiochemistryBacteriaMembrane

Abstract

fetched live from OpenAlex

The present work seeks to determine the impact of weight percentage (wt%) of grafted starch nanocrystals (g-SNCs) on the oxygen and water vapour permeability of poly (lactic acid), PLA. Changes in the oxygen and water vapour permeability of PLA due to changes in PLA's crystalline structures and lamellar thickness were quantified. To this end, 3, 5, and 7 wt% of g-SNC nanoparticles were blended with PLA using the solvent casting method in order to study impact of g-SNC nanoparticles on crystallization behaviour, long spacing period, melting behavior, and oxygen and water barrier properties of PLA nanocomposites. This was achieved by wide-angle X-ray diffraction (WAXD), small-angle X-ray diffraction (SAXD), differential scanning calorimetry (DSC), and oxygen and water vapour permeability machine. The results of the WAXD and SAXD analysis show that the addition of 5 wt% g-SNC in PLA induces α crystal structure at a lower crystallization time, while it significantly increases the α crystal thickness of PLA, in comparison to neat PLA. However, when g-SNC concentrations were altered (i.e., 3 or 7 wt%), the crystallization time was found to increase due to the thermodynamic barrier of crystallization. Finally, the oxygen and water vapour permeability of PLA/SNC-g-LA (5 wt%) nanocomposite film were found to be reduced by ∼70% and ~50%, respectively, when compared to the neat PLA film. This can lead to the development of PLA nanocomposites with high potential for applications in food packaging.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.081
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.231
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it