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Record W4285612169 · doi:10.1039/d2nr02714c

Solution combustion synthesis: the relevant metrics for producing advanced and nanostructured photocatalysts

2022· review· en· W4285612169 on OpenAlexaff
Fizza Siddique, Sergio González-Cortés, Amir Mirzaei, Tiancun Xiao, M. A. Rafiq, Xiaoming Zhang

Bibliographic record

VenueNanoscale · 2022
Typereview
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsInstitut National de la Recherche Scientifique
FundersNational Natural Science Foundation of ChinaUniversity of Oxford
KeywordsCombustionPhotocatalysisMaterials scienceNanotechnologyProcess engineeringProduct (mathematics)Computer scienceBiochemical engineeringCatalysisChemistryEngineeringMathematicsOrganic chemistry

Abstract

fetched live from OpenAlex

green and sustainable paths to accomplish chemical circularity. The design and preparation methods of photocatalysts play a prime role in determining the structural, surface characteristics and optoelectronic properties of the final products. The solution combustion synthesis (SCS) technique is a relatively novel, cost-effective, and efficient method for the bulk production of nanostructured materials. SCS-fabricated metal oxides are of great technological importance in photocatalytic, environmental and energy applications. To date, the SCS route has been employed to produce a large variety of solid materials such as metals, sulfides, carbides, nitrides and single or complex metal oxides. This review intends to provide a holistic perspective of the different steps involved in the chemistry of SCS of advanced photocatalysts, and pursues several SCS metrics that influence their photocatalytic performances to establish a feasible approach to design advanced photocatalysts. The study highlights the fundamentals of SCS and the importance of various combustion parameters in the characteristics of the fabricated photocatalysts. Consequently, this work deals with the design of a concise framework to link the fine adjustment of SCS parameters for the development of efficient metal oxide photocatalysts for energy and environmental applications.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.002
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.002
Science and technology studies0.0000.001
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.038
GPT teacher head0.312
Teacher spread0.274 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations138
Published2022
Admission routes1
Has abstractyes

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