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Record W4289861516 · doi:10.1111/php.13686

Exploring the Antibacterial Properties of Lignin‐coated Magnetic Nanoparticles Synthesized in a One‐pot Process<sup>†</sup>

2022· article· en· W4289861516 on OpenAlexafffund
Daliane R. C. da Silva, J. C. Scaiano

Bibliographic record

VenuePhotochemistry and Photobiology · 2022
Typearticle
Languageen
FieldMaterials Science
TopicAdvanced Nanomaterials in Catalysis
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsBiocompatibilityNanomaterialsAntibacterial activityLigninNanocompositeNanotechnologyMaterials scienceIrradiationNanoparticleCoatingChemistryChemical engineeringOrganic chemistryBacteria

Abstract

fetched live from OpenAlex

Given the current grave problems with antibiotic resistance, the discovery of novel, unconventional antibacterial drugs is not just important but also urgent. In this contribution, we report on the synthesis and testing of several composite nanomaterials that may find applications as therapeutic drugs or surface disinfectants. These materials are based on magnetic nanostructures coated with lignin, for example, lignin@FeCo. The magnetic properties of these nanocomposites facilitate removal or localization, whereas the lignin shell provides biocompatibility. These nanomaterials are mild antibacterials in the absence of light, but when illuminated become powerful antibacterial agents with typically ≥6 log units of bacterial reduction in 1-5 min of irradiation. These materials are strongly absorbing, including in the very useful NIR biological window, which we illustrate using 810 nm LED irradiation. We also show that in the short time required for antibacterial action, thermal changes are very small (≤5°C). Further, biocompatibility tests using fibroblasts show very limited cell damage and no enhanced adverse effect during 810 nm NIR illumination. As a surface coating for the active material, lignin provides a "trojan horse" strategy to facilitate the antibacterial action.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.659

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.053
GPT teacher head0.238
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2022
Admission routes2
Has abstractyes

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