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Record W4291805246 · doi:10.21203/rs.3.rs-1898174/v1

Arsenic removal performance of granular adsorbents using novel clinoptilolites modified with iron nanoparticles

2022· preprint· en· W4291805246 on OpenAlexaff
Shamin Hosseini Nami, Seyed Borhan Mousavi, Sara Fazli-Shokouhi, M. Khatamian

Bibliographic record

VenueResearch Square · 2022
Typepreprint
Languageen
FieldEnvironmental Science
TopicArsenic contamination and mitigation
Canadian institutionsUniversity of British Columbia
Fundersnot available
KeywordsAdsorptionChitosanBeadNuclear chemistryArsenicSodium alginateFreundlich equationChemistryClinoptiloliteSodium hydroxideChromatographyMaterials scienceSodiumZeoliteOrganic chemistryCatalysisComposite material

Abstract

fetched live from OpenAlex

Abstract In this research, novel beads were successfully synthesized from natural clinoptilolite (CL) modified with iron nanoparticles (FCL). Beads were prepared using alginate (A) and chitosan (C). FESEM, EDX, XRD, and FTIR techniques were employed to characterize the CL, FCL, A-bead, and C-bead. A comprehensive series of batch adsorption experiments were conducted utilizing both prepared samples to study the influential parameters. The most effective cross-linking solutions of chitosan and alginate were sodium tripolyphosphate/sodium hydroxide and 4% Ferric chloride, respectively. The optimum ratio of chitosan/FCL and alginate/FCL was 1:3 and 1:4, sequentially. The effect of initial arsenic concentration, and adsorbent concentration were evaluated. The optimal removal rate of 86% and 93.27% were found for A-beads and C-beads using their optimized initial concentration. Moreover, the best arsenic removal performance was seen 1 g/L for both A-beads and C-beads. The removal rate of 0.3, 0.6, 1, 1.5, and 2 g/L of alginate was 75.12%, 81.15%, 82.21%, 82.90%, and 83.15%, respectively. On the other hand, C-beads had higher removal rates at the considered contents. The removal rate of 0.3, 0.6, 1, 1.5, and 2 g/L of C-beads were 75.18%, 88.78%, 91.86%, 92.25%, and 92.4%, respectively. Additionally, Langmuir and Freundlich isotherms were employed to find the maximum adsorption capacity. The maximum adsorption capacity of qmax of alginate and chitosan beads was 10000 𝜇g/g.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.073
GPT teacher head0.348
Teacher spread0.275 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2022
Admission routes1
Has abstractyes

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