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Record W4292099386 · doi:10.1002/cjce.24605

Use of <scp> O <sub>3</sub> </scp> and <scp> O <sub>3</sub> </scp> / <scp> H <sub>2</sub> O <sub>2</sub> </scp> for degradation of organic matter from Bayer liquor towards new resource management: Kinetic and mechanism

2022· article· en· W4292099386 on OpenAlexvenueno aff
Miguel Antonio Soplin Pastor, Amilton Barbosa Botelho, Jorge Alberto Soares Tenório, Denise Crocce Romano Espinosa, Marcela dos Passos Galluzzi Baltazar

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2022
Typearticle
Languageen
FieldEngineering
TopicBauxite Residue and Utilization
Canadian institutionsnot available
FundersUniversidade de São PauloFundação de Amparo à Pesquisa do Estado de São Paulo
KeywordsOrganic matterTotal organic carbonChemistryOxalateDegradation (telecommunications)OzoneNuclear chemistryEnvironmental chemistryInorganic chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Since the quality of bauxite resources has decreased and the organic carbon content has increased, different approaches are explored to remove the organic matter in alumina production. Advanced oxidative processes (AOPs) represent a possibility since they are widely used as an alternative for treating wastewaters to degrade organic pollutant molecules and in hydrometallurgy processes. For this reason, the goal of the project was the ozonation of Bayer liquor for organic matter removal. The ozone concentration was evaluated over time, as well as the H 2 O 2 concentration and temperature. Results showed that the total organic carbon (TOC) removal achieved 19% in the most optimized condition with a kinetic rate of 0.0157 h −1 –21.9 mg/L O 3 , 0.05 mol/L H 2 O 2 at 80°C. The colour of the liquor changed from dark brown to white‐yellow, indicating that the size of the organic compounds had decreased. Also, 95.4% of degraded TOC formed CO 2 , and almost 50% of the organic matter was oxalate compounds. The energy required for ozone production versus removed organic matter demonstrated that the technique proposed might be technically and economically feasible to be applied in the Bayer process. The study demonstrates the application of AOP in an extremely alkaline condition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.174
Teacher spread0.164 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2022
Admission routes1
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical EngineeringSame topicBauxite Residue and UtilizationFrench-language works237,207