MétaCan
Menu
Back to cohort
Record W4296689036 · doi:10.1021/jacsau.2c00424

Activity Self-Optimization Steered by Dynamically Evolved Fe<sup>3+</sup>@Fe<sup>2+</sup> Double-Center on Fe<sub>2</sub>O<sub>3</sub> Catalyst for NH<sub>3</sub>-SCR

2022· article· en· W4296689036 on OpenAlex
Hai Yang Yuan, Ningning Sun, Jianfu Chen, Hua Gui Yang, P. Hu, Haifeng Wang

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueJACS Au · 2022
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsnot available
FundersNational Ten Thousand Talent ProgramFundamental Research Funds for the Central UniversitiesNational Key Research and Development Program of ChinaEast China University of Science and TechnologyMinistry of Science and Technology of the People's Republic of ChinaCentral University Basic Research Fund of ChinaQueen's UniversityNational Natural Science Foundation of China
KeywordsCatalysisActive centerIn situCenter (category theory)ChemistrySteady state (chemistry)Materials scienceNanotechnologyPhysical chemistryCrystallographyOrganic chemistry

Abstract

fetched live from OpenAlex

-SCR at middle-high temperatures instead of high temperatures. Our findings demonstrate the atomic-level self-evolution of active sites and the dynamically adjusted activity variation of the catalyst under the in-situ condition during the reaction process and provide insights into the reaction mechanism and catalyst optimization.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.076
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.001
Meta-epidemiology (narrow)0.0020.002
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0010.002
Science and technology studies0.0020.001
Scholarly communication0.0010.002
Open science0.0030.002
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.234
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it