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Starch-Stabilized Iron Oxide Nanoparticles for the Photocatalytic Degradation of Methylene Blue

2022· article· en· W4296742967 on OpenAlexafffund
Natun Dasgupta, Milind Ajith Nayak, Mario Gauthier

Bibliographic record

VenuePolysaccharides · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicAdvanced oxidation water treatment
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPhotocatalysisCatalysisStarchHydrogen peroxideChemistryMethylene blueAqueous solutionNanoparticleIron oxideIron oxide nanoparticlesDegradation (telecommunications)Inorganic chemistryChemical engineeringOrganic chemistry

Abstract

fetched live from OpenAlex

The photocatalytic Fenton process, which produces a strong oxidant in the form of hydroxyl radicals, is a useful method to degrade organic contaminants in water. The Fenton reaction uses hydrogen peroxide and Fe2+ ions under relatively acidic conditions (typically pH 2–3) to maintain solubility of the iron catalyst but is troublesome due to the large volumes of decontaminated yet highly acidic water generated. Starch-stabilized iron (Fe2+/Fe3+) oxide nanoparticles were synthesized to serve as a colloidal catalyst system as the hydrophilic starch effectively prevents precipitation of the nanoparticles under conditions closer to neutrality. To evaluate the usefulness of this catalyst system for the photo-Fenton degradation of methylene blue as a model dye, the preparation protocol used and the iron loading in the starch were varied. The photocatalytic Fenton reaction was investigated at pH values up to 4. Not only were the starch-stabilized catalysts able to decolorize the dye but also to mineralize it in part, that is, to degrade it to carbon dioxide and water. The catalysts could be reused in several degradation cycles. This demonstrates that starch is an efficient stabilizer for iron oxide nanoparticles in aqueous media, enabling their use as environmentally friendly and cost-effective photo-Fenton catalysts. These starch-stabilized iron nanoparticles may also be useful to degrade other dyes and pollutants in water, such as pesticides.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.020
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.260
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2022
Admission routes2
Has abstractyes

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