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Influence of an atomic resonance on the coherent control of the photoionization process

2022· article· en· W4296844519 on OpenAlexafffund
Elena V. Gryzlova, Paolo Carpeggiani, Maria M. Popova, Maksim D. Kiselev, Nicolas Douguet, Maurizio Reduzzi, M. Negro, Antoine Comby, H. Ahmadi, V. Wanie, Mattea Carmen Castrovilli, Andreas Fischer, P. Johnsson, Michael Meyer, Klaus Bartschat, S. M. Burkov, Tamás Csizmadia, Mathieu Dumergue, S. Kühn, N. G. Harshitha, Miklós Füle, F. Aeenehvand, F. Stienkemeier, Denys Iablonskyi, Kiyoshi Ueda, P. Finetti, Marco Zangrando, Nicola Mahne, Kenichi L. Ishikawa, Oksana Plekan, Kevin C. Prince, E. Allaria, L. Giannessi, Carlo Callegari, Alexei N. Grum-Grzhimailo, G. Sansone

Bibliographic record

VenuePhysical Review Research · 2022
Typearticle
Languageen
FieldPhysics and Astronomy
TopicLaser-Matter Interactions and Applications
Canadian institutionsInstitut National de la Recherche Scientifique
FundersCore Research for Evolutional Science and TechnologyNatural Sciences and Engineering Research Council of CanadaJapan Society for the Promotion of ScienceMinistry of Education, Culture, Sports, Science and TechnologyFonds de Recherche du Québec-Société et CultureAlbert-Ludwigs-Universität FreiburgFonds de recherche du Québec – Nature et technologiesDeutsche ForschungsgemeinschaftNational Science Foundation
KeywordsPhotoionizationAtomic physicsNeonCoherent controlExcited stateResonance (particle physics)AmplitudePhysicsPhotoelectric effectPhotonPhoton energyPhase (matter)ExcitationLaserOpticsQuantum mechanicsIonizationIon

Abstract

fetched live from OpenAlex

In coherent control schemes, pathways connecting an initial and a final state can be independently controlled by manipulating the complex amplitudes of their transition matrix elements. For paths characterized by the absorption of multiple photons, these quantities depend on the magnitude and phase between the intermediate steps, and are expected to be strongly affected by the presence of resonances. We investigate the coherent control of the photoemission process in neon using a phase-controlled two-color extreme ultraviolet pulse with frequency in proximity of an excited energy state. Using helium as a reference, we show that the presence of such a resonance in neon modifies the amplitude and phase of the asymmetric emission of photoelectrons. Theoretical simulations based on perturbation theory are in fair agreement with the experimental observations.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.585
Threshold uncertainty score0.305

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.035
GPT teacher head0.407
Teacher spread0.372 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2022
Admission routes2
Has abstractyes

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