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Record W4297193057 · doi:10.3390/electrochem3040040

Effect of Components and Operating Conditions on the Performance of PEM Electrolyzers: A Review

2022· review· en· W4297193057 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueElectrochem · 2022
Typereview
Languageen
FieldEnergy
TopicHybrid Renewable Energy Systems
Canadian institutionsUniversity of Waterloo
FundersWaterloo Institute for Nanotechnology, University of Waterloo
KeywordsPolymer electrolyte membrane electrolysisElectrolysisProton exchange membrane fuel cellHigh-pressure electrolysisPower to gasElectrolysis of waterHigh-temperature electrolysisHydrogen productionMaterials scienceAlkaline water electrolysisElectrolyteElectrolytic cellElectrocatalystHydrogenPassivationMembrane electrode assemblyChemical engineeringProcess engineeringChemistryNanotechnologyElectrodeFuel cellsEngineeringElectrochemistry

Abstract

fetched live from OpenAlex

Hydrogen is considered to be the fuel of the future and with the advancement of fuel cell technology, there is a renewed interest in hydrogen production by the electrolysis of water. Among low-temperature water electrolysis options, polymer electrolyte membrane (PEM) electrolyzer is the preferred choice due to its compact size, intermittent use, and connectivity with renewable energy. In addition, it is possible to generate compressed hydrogen directly in the PEM electrolyzer, thereby reducing the additional pressurization cost for hydrogen storage. The development of electrocatalysts for oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) is a major focus of electrolysis research. Other components, such as PEMs, gas diffusion layers (GDL), and bipolar plates (BPs) have also received significant attention to enhance the overall efficiency of PEM electrolyzers. Improvements in each component or process of the PEM electrolyzer have a significant impact on increasing the energy efficiency of the electrolyzer. This work discusses various synthesis techniques to improve the dispersion of OER electrocatalyst and reducing catalyst loading for the PEM electrolyzer. Various techniques are discussed for the development of electrocatalysts, including nanostructured, core shell, and electrodeposition to deposit catalysts on GDL. The design and methodology of new and improved GDL are discussed along with the fabrication of gas diffusion electrodes and passivation techniques to reduce the oxidation of GDL. The passivation technique of BPs using Au and Pt is summarized for its effect on electrolysis efficiency. Finally, the optimization of various operating conditions for PEM electrolyzer are reviewed to improve the efficiency of the electrolyzer.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.955
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0020.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.292
Teacher spread0.268 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it