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Record W4297238014 · doi:10.1139/cjc-2021-0342

Novel photocatalyst system to deep desulfurization of petroleum model and gas condensate by Box–Behnken design

2022· article· en· W4297238014 on OpenAlexvenueno aff
Ilnaz Raeisi, Pirouz Derakhshi, Parviz Aberoomand Azar, Mohammad Saber Tehrani

Bibliographic record

VenueCanadian Journal of Chemistry · 2022
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsnot available
Fundersnot available
KeywordsDibenzothiopheneBox–Behnken designFlue-gas desulfurizationCatalysisPhotocatalysisTitanium dioxideChemistryFourier transform infrared spectroscopyNuclear chemistryMolybdenumScanning electron microscopeSpectroscopyChemical engineeringDiffuse reflectance infrared fourier transformNickelResponse surface methodologyAnalytical Chemistry (journal)Inorganic chemistryMaterials scienceComposite materialOrganic chemistryChromatography

Abstract

fetched live from OpenAlex

In this research, cobalt (Co)/molybdenum (Mo) and nickel (Ni) doped with titanium dioxide (TiO 2 ) were loaded onto multi-walled carbon nanotubes (MWCNTs). Then, the magnetization catalyst, iron oxide (Fe 3 O 4 ), was loaded on them, which was used for the deep desulfurization of dibenzothiophene (DBT). These catalysts were characterized by X-ray diffraction, Fourier transform infrared spectroscopy, scanning electron microscopy, energy-dispersive X-ray spectroscopy, differential reflectance spectroscopy, and Brunauer–Emmett–Teller, Barrett–Joyner–Halenda, and vibrating sample magnetometer techniques. The photocatalytic activity of these catalysts was experienced under visible light using DBT. The response surface methodology based on the Box–Behnken design was used to evaluate parameters, including catalyst dosage (g), time (min), and concentration of DBT (mg L −1 ). The highest degradation efficiency under optimal conditions for CoMoNi/TiO 2 /MWCNTs/Fe 3 O 4 catalysts with a catalyst dosage of 0.3 g, a time of 180 min, and a concentration of 50 mg L −1 was 99.99%. Optimum conditions were studied for desulfurization of the gas condensate. The highest desulfurization efficiency (90.33%) was obtained by the CoMoNi/TiO 2 /MWCNTs/Fe 3 O 4 catalyst.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.169
Threshold uncertainty score0.537

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.178
Teacher spread0.169 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2022
Admission routes1
Has abstractyes

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