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Record W4297831345 · doi:10.1007/s13762-022-04300-x

Methods and benefits of measuring non-hydrocarbon gases from surface casing vents

2022· article· en· W4297831345 on OpenAlexafffund
Nicholas Utting, Kirk Osadetz, Thomas H. Darrah, Matthias Brennwald, Bernhard Mayer, Don C. Lawton

Bibliographic record

VenueInternational Journal of Environmental Science and Technology · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsUniversity of CalgaryCarbon Management CanadaNatural Resources Canada
FundersNatural Resources CanadaOffice of Energy Research and DevelopmentGovernment of Canada
KeywordsMethaneNoble gasCasingNatural gasMass spectrometryChemistryArgonHydrocarbonGas chromatographyGroundwaterQuadrupole mass analyzerTrace gasNatural gas fieldEnvironmental chemistryIsotope-ratio mass spectrometryAnalytical Chemistry (journal)Atmosphere (unit)GeologyPetroleum engineeringChromatographyPhysicsMeteorology

Abstract

fetched live from OpenAlex

Abstract Surface casing vents divert natural gas migration along oil and gas boreholes to bypass groundwater, with the gas venting to the atmosphere. While this strategy is designed to protect groundwater, it constitutes a source of greenhouse gases to the atmosphere. In instances where gas leakage occurs, the characterization of the molecular and isotopic composition of natural gas emitted from surface casing vent flows can be used to assist in identifying the gas source. We compare concentration measurements of non-hydrocarbon gases (within natural gas) of samples analyzed by laboratory-based gas chromatography (N 2 , Ar, CO 2 and O 2 ) and magnetic sector noble gas mass spectrometry (He, Ar and Kr) with field measurements conducted using a field portable quadrupole mass spectrometer (miniRUEDI). The standard deviation of miniRUEDI concentration results was within plus/minus one standard deviation of samples measured using laboratory-based GC (N 2 , O 2 , Ar and He) and magnetic sector noble gas mass spectrometry (He, Ar). Additional laboratory-based determination of isotope ratios of methane and argon (δ 13 C CH4 , δ 2 H CH4 , and 40 Ar/ 36 Ar) enabled a comparison between information provided by the analysis of reactive gases compared with noble gas isotopes. Gases from different sources displayed quantifiable differences in δ 13 C CH4 and δ 2 H CH4 , but these changes may or may not be distinguished if only one sampling event is conducted. By comparison, 40 Ar/ 36 Ar further enabled the differentiation of various gas sources. The objective of this paper is to discuss the advantages and trade-offs of the three different analysis methods considered, and the feasibility of their application in different environmental monitoring scenarios.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.483
Threshold uncertainty score0.449

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.246
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2022
Admission routes2
Has abstractyes

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