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Record W4300961429 · doi:10.1002/app.53177

Structure change of atactic polystyrene upon aging

2022· article· en· W4300961429 on OpenAlexaff
Ahmed Abdeldaym, Ralf Brüning

Bibliographic record

VenueJournal of Applied Polymer Science · 2022
Typearticle
Languageen
FieldMaterials Science
TopicMaterial Dynamics and Properties
Canadian institutionsMount Allison University
FundersMinistry of Higher Education
KeywordsPolystyreneMaterials sciencePolymer sciencePolymer chemistryComposite materialPolymer

Abstract

fetched live from OpenAlex

Abstract We report the changes of atactic polystyrene (a‐PS) upon annealing below the glass transition based on X‐ray scattering, volume, and differential scanning calorimetry measurements of samples in the quenched and annealed states. Upon relaxation, an increase of the main diffuse diffraction peak and a decrease of the polymerization peak, typical for a‐PS, are proportional to the enthalpy changes. The relaxation of enthalpy corresponds to a change of the fictive temperature by 6.1 K for annealing at 80°C for 24 h. The changes of the fictive temperature derived from the X‐ray structure factor are between 5.4 and 6.8 K, depending on the range of scattering vector. The relaxation signal has a zero crossing at low scattering angles. The volume of the samples, measured at ambient conditions, did not change upon relaxation. We attribute these observations to localized relaxation processes that involve a small number of phenyl groups.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.233
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2022
Admission routes1
Has abstractyes

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