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Record W4303857808 · doi:10.1002/sscp.202200104

Beta‐cyclodextrin covalent organic framework coated silica composite as chiral stationary phase for high‐performance liquid chromatographic separation

2022· article· en· W4303857808 on OpenAlexaff
Yilun Yan, Xinting Cai, Siyuan Cheng, Xue-Xian Xie, Yixin Lan, Shuanghao Wu, Jun Fan, Sheng‐Run Zheng, Song‐Liang Cai, Wei‐Guang Zhang

Bibliographic record

VenueSeparation Science Plus · 2022
Typearticle
Languageen
FieldMaterials Science
TopicCovalent Organic Framework Applications
Canadian institutionsInstitute of Aging
FundersNatural Science Foundation of Guangdong ProvinceNational Natural Science Foundation of China
KeywordsCyclodextrinCovalent bondHigh-performance liquid chromatographyChromatographyCovalent organic frameworkChemistryPhase (matter)Chiral column chromatographyColumn chromatographyBeta-CyclodextrinsComposite numberOrganic chemistryMaterials science

Abstract

fetched live from OpenAlex

Abstract A beta‐cyclodextrin covalent organic framework coated silica composite, namely beta‐cyclodextrin covalent organic framework@SiO 2 , was prepared by coating the beta‐cyclodextrin covalent organic framework onto a spherical aminized silica matrix and used as the chiral stationary phase for high‐performance liquid chromatography separation in both normal‐ and reversed‐phase modes. The beta‐cyclodextrin covalent organic framework@SiO 2 packed column showed good separation performance towards positional isomers such as nitrotoluene and aminophenol, and benzene homologs in the reversed‐phase high‐performance liquid chromatography mode. While chiral drug molecules including omeprazole and lansoprazole could be also enantioseparated on beta‐cyclodextrin covalent organic framework@SiO 2 packed column in the normal‐phase high‐performance liquid chromatography mode. Besides, the effects of mobile phase composition, column temperature, and other factors of high‐performance liquid chromatography separation on beta‐cyclodextrin covalent organic framework@SiO 2 packed column were studied in detail. Moreover, the stability test of the beta‐cyclodextrin covalent organic framework@SiO 2 packed column was also investigated. The results of continuous injections and monthly detection were basically identical, suggesting the excellent durability of the obtained high‐performance liquid chromatography column. This work indicated that beta‐cyclodextrin covalent organic framework@SiO 2 composite could effectively separate different compounds in high‐performance liquid chromatography normal/reversed‐phase modes, making it a promising chiral stationary phase in the field of high‐performance liquid chromatography separation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.338
Teacher spread0.317 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2022
Admission routes1
Has abstractyes

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