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Record W4304083996 · doi:10.1063/5.0120169

Equation of state of solid parahydrogen using <i>ab initio</i> two-body and three-body interaction potentials

2022· article· en· W4304083996 on OpenAlexafffund
Alexander Ibrahim, Pierre–Nicholas Roy

Bibliographic record

VenueThe Journal of Chemical Physics · 2022
Typearticle
Languageen
FieldPhysics and Astronomy
TopicQuantum, superfluid, helium dynamics
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsSpin isomers of hydrogenMonte Carlo methodExtrapolationInteraction energyPath integral Monte CarloAb initioAb initio quantum chemistry methodsStatistical physicsPhysicsChemistryQuantum Monte CarloHydrogenMathematicsQuantum mechanicsMathematical analysis

Abstract

fetched live from OpenAlex

at T = 4.2 K, calculated using path integral Monte Carlo simulations, with ab initio two-body and three-body interaction potentials. We correct for finite size simulation errors using potential tail corrections. Trotter factorization errors are accounted for either via extrapolation or by using a suitably small imaginary time step. We incorporate the three-body interaction using two methods: (1) the full inclusion method, where pair and three-body interactions are used in both Monte Carlo sampling and in the energy estimators, and (2) the perturbative method, where three-body interactions are omitted from sampling but are still present in energy estimations. Both treatments of the three-body interaction return very similar total energies and pressures. The presence of three-body interactions has only minor effects on the structural properties of the solid. Whereas the pair interaction, on its own, significantly overestimates the pressure of solid parahydrogen, the additional presence of the three-body interaction causes a severe underestimation of the pressure. Our findings suggest that accurate simulations of solid parahydrogen require four-body and possibly higher-order many-body interactions. It may also be the case that static interaction potentials are entirely unsuitable for simulations of solid parahydrogen at high densities.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.214
Threshold uncertainty score0.427

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.285
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2022
Admission routes2
Has abstractyes

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