High Permittivity Polymer Composites on the Basis of Long Single-Walled Carbon Nanotubes: The Role of the Nanotube Length
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Bibliographic record
Abstract
Controlling the permittivity of dielectric composites is critical for numerous applications dealing with matter/electromagnetic radiation interaction. In this study, we have prepared polymer composites, based on a silicone elastomer matrix and Tuball carbon nanotubes (CNT) via a simple preparation procedure. The as-prepared composites demonstrated record-high dielectric permittivity both in the low-frequency range (102−107 Hz) and in the X-band (8.2−12.4 GHz), significantly exceeding the literature data for such types of composite materials at similar CNT content. Thus, with the 2 wt% filler loading, the permittivity values reach 360 at 106 Hz and >26 in the entire X-band. In similar literature, even the use of conductive polymer hosts and various highly conductive additives had not resulted in such high permittivity values. We attribute this phenomenon to specific structural features of the used Tuball nanotubes, namely their length and ability to form in the polymer matrix percolating network in the form of neuron-shaped clusters. The low cost and large production volumes of Tuball nanotubes, as well as the ease of the composite preparation procedure open the doors for production of cost-efficient, low weight and flexible composites with superior high permittivity.
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Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.002 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.001 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.001 | 0.001 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.002 | 0.001 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.006 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it