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Ultrasonically synthesized MOFs for modification of polymeric membranes: A critical review

2022· review· en· W4306252716 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueUltrasonics Sonochemistry · 2022
Typereview
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaCanada's Oil Sands Innovation AllianceAlberta Innovates
KeywordsMembraneSonicationMaterials scienceSurface modificationSonochemistryNanotechnologyChemical engineeringGas separationMetal-organic frameworkOrganic chemistryChemistryAdsorptionEngineering

Abstract

fetched live from OpenAlex

Metal-organic framework (MOF) membranes hold the promise for energy-efficient separation processes. These nanocrystalline compounds can effectively separate materials with different sizes and shapes at a molecular level. Furthermore, MOFs are excellent candidates for improving membrane permeability and/or selectivity due to their unique properties, such as high specific area and special wettability. Generally, MOFs can be used as fillers in mixed matrix membranes (MMMs) or incorporated onto the membrane surface to modify the top layer. Characteristics of the MOFs, and correspondingly, the properties of the MOF-based membranes, are majorly affected by their production technique. This critical review discusses the sonication technique for MOF production and the opportunities and challenges of using MOF for making membranes. Effective parameters on the characteristics of the synthesized MOFs, such as sonication time and power, were discussed in detail. Although the ultrasonically synthesized MOFs have shown great potential in the fabrication/modification of membranes for gas and liquid separation/purification, so far, no comprehensive and critical review has been published to clarify such accomplishments and technological gaps for the future research direction. This paper aims to review the most recent research conducted on ultrasonically synthesized MOF for the modification of polymeric membranes. Recommendations are provided with the intent of identifying the potential future works to explore the influential sonication parameters.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.010
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMetaresearch, Meta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.944
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.010
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0040.002
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0020.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0140.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.071
GPT teacher head0.343
Teacher spread0.272 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it