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Record W4307820327 · doi:10.1002/cjce.24746

Heterogeneous catalyzed isomerization of turpentine oil by ordered mesoporous materials like M41S structures

2022· article· en· W4307820327 on OpenAlexvenueno aff
Leonardo Borges de Sousa, Jessica T. Speranza, Rodrigo Condotta, Rodrigo Cella

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2022
Typearticle
Languageen
FieldMaterials Science
TopicMesoporous Materials and Catalysis
Canadian institutionsnot available
FundersFundação de Amparo à Pesquisa do Estado de São Paulo
KeywordsIsomerizationCampheneMesoporous materialCatalysisMolecular sieveHeteroatomMCM-41ChemistryTurpentineOrganic chemistryChemical engineeringMaterials scienceChromatographyEssential oil

Abstract

fetched live from OpenAlex

Abstract Herein, the synthesis of a structure with a porous system similar to that of molecular sieves, MCM‐41 and 48 types, with the incorporation of heteroatoms in their synthesis, is reported. The catalytic activity of these materials was tested in the isomerization reaction of turpentine oil to obtain camphene. The best results were obtained with Zn‐Al‐Si‐MCM, a mesoporous material, with a conversion of up to 96% and selectivities of 31% and 22% to camphene and 4‐carene, respectively, both of which are bicyclic products. The recycling of the catalyst was also tested, and after three cycles, no significant loss of activity was observed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.176
Teacher spread0.171 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2022
Admission routes1
Has abstractyes

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