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Record W4307871226 · doi:10.3389/fphot.2022.1037473

Upconverting nanoparticles as primary thermometers and power sensors

2022· article· en· W4307871226 on OpenAlexafffund
Joana Costa Martins, Artiom Skripka, Carlos D. S. Brites, Antonio Benayas, Rute A. S. Ferreira, Fiorenzo Vetrone, Luís D. Carlos

Bibliographic record

VenueFrontiers in Photonics · 2022
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsInstitut National de la Recherche Scientifique
FundersFonds de recherche du Québec – Nature et technologiesCentro de Investigação em Materiais Cerâmicos e CompósitosFundação para a Ciência e a TecnologiaMinisterio de Economía y CompetitividadComunidad de Madrid
KeywordsLuminescenceLaserNanosensorMaterials scienceExcitationNanoparticleOptoelectronicsPhosphorLaser power scalingNanotechnologyAnalytical Chemistry (journal)ChemistryOpticsPhysics

Abstract

fetched live from OpenAlex

Luminescence thermometry is a spectroscopic technique for remote temperature detection based on the thermal dependence of the luminescence of phosphors, presenting numerous applications ranging from biosciences to engineering. In this work, we use the Er 3+ emission of the NaGdF 4 /NaGdF 4 :Yb 3+ ,Er 3+ /NaGdF 4 upconverting nanoparticles upon 980 nm laser excitation to determine simultaneously the absolute temperature and the excitation power density. The Er 3+ 2 H 11/2 → 4 I 15/2 and 4 S 3/2 → 4 I 15/2 emission bands, which are commonly used for thermometric purposes, overlap with the 2 H 9/2 → 4 I 13/2 emission band, which can lead to erroneous temperature readout. Applying the concept of luminescent primary thermometry to resolve the overlapping Er 3+ transitions, a dual nanosensor synchronously measuring the temperature and the delivered laser pump power is successfully realized holding promising applications in laser-supported thermal therapies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.205
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2022
Admission routes2
Has abstractyes

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Same venueFrontiers in PhotonicsSame topicLuminescence Properties of Advanced MaterialsFrench-language works237,207