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Record W4308435051 · doi:10.1021/acsanm.2c04050

Self-Powered Humidity Sensors Based on SnS<sub>2</sub> Nanosheets

2022· article· en· W4308435051 on OpenAlexaff
Leyla Shooshtari, Nassim Rafiefard, Maryam Barzegar, Somayeh Fardindoost, Azam Iraji zad, Raheleh Mohammadpour

Bibliographic record

VenueACS Applied Nano Materials · 2022
Typearticle
Languageen
FieldEngineering
TopicAdvanced Sensor and Energy Harvesting Materials
Canadian institutionsUniversity of Victoria
FundersIran National Science FoundationSharif University of Technology
KeywordsMaterials scienceHumidityTriboelectric effectNanosheetOptoelectronicsSubstrate (aquarium)NanotechnologyTin oxideChemical vapor depositionDielectricAdsorptionComposite materialDopingChemistry

Abstract

fetched live from OpenAlex

With the advent of the Internet of Things (IoT), the development of self-powered sensors has received much attention. Introducing triboelectric nanogenerators (TENGs) as a power source that converts mechanical movement into electrical signals has been admired recently. Moreover, the monitoring of humidity has become enormously essential in several technological contexts from environment monitoring to biomedical applications, thus joining these two subjects provides a huge benefit in achieving self-powered humidity sensors. Here, in this research, facile, low-priced and self-powered humidity sensors are fabricated utilizing transition-metal dichalcogenides (TMD) nanosheets. Semi-vertical SnS2 nanosheets are synthesized through a modified chemical vapor deposition method at moderate heat treatment (500 °C) utilizing pristine sensor’s substrate and sulfur element on a laser grooved fluorine tin-doped oxide (FTO)/glass. To achieve a self-powered device, the integrated contact-separated (CS) TENG of FTO and Kapton/Al has been coupled with the projected humidity sensor, through the impedance matching circuit. This self-powered SnS2 humidity sensor demonstrated an outstanding response of about 400%, fast response and recovery times (∼4, and 7 s), and long-term stability (at least 5 months). Furthermore, the humidity effect on the electrical performance of the SnS2 layer was studied through first-principle simulations. Based on calculated adsorption energies, charge transfer, electronic band structures, and density of states, H2O molecules physisorbed on the SnS2 nanosheet with a strong adsorption energy of −1.82 eV and 0.0208 e/molecule charges transferred from H2O molecules to the surface. Our density functional theory calculations shed light on the humidity sensing mechanism by illustrating that both Sn and Sulfur atoms could act as adsorption sites. The introduced battery-free and self-powered humidity sensors have great conceivable application in wearable/portable electronics and also smart homes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.134
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.192
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations32
Published2022
Admission routes1
Has abstractyes

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