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Record W4308645685 · doi:10.1002/cjce.24760

An optimization study for preventing silica gelation and improving filtration effectiveness during <scp>pH</scp> reduction of high concentration silica solutions

2022· article· en· W4308645685 on OpenAlexafffundvenue
Saheli Rao, S. Murugan, Gopal Achari, Basil Perdicakis, Anil K. Mehrotra

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2022
Typearticle
Languageen
FieldEnvironmental Science
TopicCO2 Sequestration and Geologic Interactions
Canadian institutionsSuncor Energy (Canada)University of Calgary
FundersCanada's Oil Sands Innovation AllianceMitacs
KeywordsFiltration (mathematics)Response surface methodologyChromatographyChemistryWastewaterChemical engineeringMaterials scienceEnvironmental engineeringEnvironmental scienceMathematics

Abstract

fetched live from OpenAlex

Abstract The steam generation processes at the steam‐assisted gravity drainage facilities result in huge quantities of wastewater streams, which are characterized by high pH and high silica levels. These concentrated streams need to be neutralized before their disposal via down‐hole injection. The neutralization of these high‐pH brines results in the formation of a gel‐like substance, which makes it difficult to filter the amorphous silica gel. The wastewater used in this study was synthetically prepared using sodium metasilicate to mimic high‐concentration silica solutions. Our experiments did not show any advantage of a two‐step pH‐neutralization process over the single‐step process for suppressing silica gelation. A systematic experimental campaign was undertaken to investigate the effects of SiO 2 concentration, NaCl:SiO 2 ratio, and pH on the residual silica concentration, percent silica removal, filtration rate, and filtration effectiveness. For NaCl:SiO 2 ratios higher than 4.5, silica precipitation during pH reduction did not lead to the formation of gel or sol. The response surface methodology (RSM), based on the Doehlert design of experiments, was implemented to optimize the responses and provide high efficacy with fewer experiments. The results from the analysis of variance (ANOVA) analyses of the experimental data were used to evaluate the significance of each term in the quadratic model. 3D response surfaces and 2D contour plots were generated for determining the optimal ranges of independent factors for achieving the maximum silica removal, the highest filtration rate, the best filtration effectiveness, and the minimum residual silica concentration. An optimum operating region was established from the RSM analysis and overlay plot.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.185
Threshold uncertainty score0.270

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.202
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations8
Published2022
Admission routes3
Has abstractyes

Explore more

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