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Record W4308766907 · doi:10.3390/polym14214693

A Simple Trick to Increase the Areal Specific Capacity of Polypyrrole Membrane: The Superposition Effect of Methyl Orange and Acid Treatment

2022· article· en· W4308766907 on OpenAlexafffund
Zahra Roohi, Frej Mighri, Ze Zhang

Bibliographic record

VenuePolymers · 2022
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsUniversité Laval
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPolypyrroleSimple (philosophy)Methyl orangeMembraneSuperposition principleOrange (colour)ChemistryMaterials sciencePolymer chemistryOrganic chemistryMathematicsBiochemistryFood sciencePolymerPolymerizationMathematical analysis

Abstract

fetched live from OpenAlex

Polypyrrole (PPy) is one of the attractive conducting polymers that have been investigated as energy storage materials in devices like supercapacitors. Previously, we have reported a free-standing soft PPy membrane synthesized through interfacial polymerization in which methyl orange (MO) and ferric chloride were used as nano template and oxidant. In this work, we report that the presence of MO and the treatment of the PPy–MO membrane with sulfuric acid can dramatically increase the specific capacitance of the membrane. The properties of the membranes were evaluated using scanning electron microscope (SEM) for morphology, Fourier transform infrared spectroscopy (FTIR) and X-ray photoelectron spectroscopy (XPS) for chemistry, thermogravimetric analysis (TGA) for thermal stability, and cyclic voltammetry (CV), and electrochemical impedance spectroscopy (EIS) for electrochemical activity. It was found that the areal specific capacitance of the PPy membrane increased from 2226 mF/cm2 to 6417 mF/cm2 and the charge transfer resistivity decreased from about 17 Ω to 3 Ω between 10,000 and 0.1 Hz due to the presence of MO and the acid treatment. It is likely that the superposition effect of MO and acid treatment helped the charge transfer process and consequently enhanced the charge storage performance and specific capacitance of the PPy membrane.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.253
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2022
Admission routes2
Has abstractyes

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