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Record W4308975790 · doi:10.1038/s41598-022-23893-4

Random lasing and replica symmetry breaking in GeO2-PbO-MgO glass–ceramics doped with neodymium

2022· article· en· W4308975790 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueScientific Reports · 2022
Typearticle
Languageen
FieldPhysics and Astronomy
TopicRandom lasers and scattering media
Canadian institutionsUniversity of Toronto
FundersInstituto Nacional de FotônicaUniversidade Federal de PernambucoConselho Nacional de Desenvolvimento Científico e TecnológicoCoordenação de Aperfeiçoamento de Pessoal de Nível Superior
KeywordsMaterials scienceCrystallinityLasing thresholdAnalytical Chemistry (journal)PhotoluminescenceNeodymiumGermanateGlass transitionDopingOpticsLaserOptoelectronicsChemistryPhysicsPolymerWavelengthComposite material

Abstract

fetched live from OpenAlex

Abstract We investigated the random lasing process and Replica Symmetry Breaking (RSB) phenomenon in neodymium ions (Nd 3+ ) doped lead-germanate glass–ceramics (GCs) containing MgO. Glass samples were fabricated by conventional melt-quenching technique and the GCs were obtained by carefully devitrifying the parent glasses at 830 °C for different time intervals. The partial crystallization of the parent glasses was verified by X-ray diffraction. Photoluminescence (PL) enhancement of $$\approx$$ <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mo>≈</mml:mo> </mml:math> 500% relative to the parent glasses was observed for samples with a higher crystallinity degree (annealed during 5 h). Powders with grains having average size of 2 µm were prepared by griding the GCs samples. The Random Laser (RL) was excited at 808 nm, in resonance with the Nd 3+ transition 4 I 9/2 → { 4 F 5/2 , 2 H 9/2 }, and emitted at 1068 nm (transition 4 F 3/2 → 4 I 11/2 ). The RL performance was clearly enhanced for the sample with the highest crystallinity degree whose energy fluence excitation threshold (EFE th ) was 0.25 mJ/mm 2 . The enhanced performance is attributed to the residence-time growth of photons inside the sample and the higher quantum efficiency of Nd 3+ incorporated within the microcrystals, where radiative losses are reduced. Moreover, the phenomenon of Replica Symmetry Breaking (RSB), characteristic of a photonic-phase-transition, was detected by measuring the intensity fluctuations of the RL emission. The Parisi overlap parameter was determined for all samples, for excitation below and above the EFE th . This is the first time, for the best of the authors knowledge, that RL emission and RSB are reported for a glass–ceramic system.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.759
Threshold uncertainty score0.588

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.207
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it