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Record W4310815762 · doi:10.1039/d2na00562j

Modeling of a two-stage polymerization considering glass fibre sizing using molecular dynamics

2022· article· en· W4310815762 on OpenAlexafffund
Lukas Schöller, Britta Nestler, Colin Denniston

Bibliographic record

VenueNanoscale Advances · 2022
Typearticle
Languageen
FieldComputer Science
TopicComputer Graphics and Visualization Techniques
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of CanadaCanadian Network for Research and Innovation in Machining Technology, Natural Sciences and Engineering Research Council of CanadaDeutsche Forschungsgemeinschaft
KeywordsSizingPolymerizationCuring (chemistry)Glass fiberMaterials scienceMolecular dynamicsComposite materialPolymerChemistryComputational chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Fibre reinforced polymers are an important class of materials due to their light weight, high strength, and stiffness. However, there is a lack of knowledge about the interaction of fibre surface, sizing (fibre coating), and resin. Often only idealised academic systems are studied, and only rarely realistic systems that are used in an industrial context. Therefore, methods for studying the behaviour of complex sizing are highly desirable, especially as they play a crucial role in the performance of fibre reinforced polymers. Here, a simplified, yet industrially used resin system is extended using molecular dynamics simulations by adding a fibre surface and sizing layers. Furthermore, a common coupling agent was selected, and several additional assumptions were made about the structure of the sizing. Based on this, a systematic procedure for the development of a final cured system is introduced: a condensation reaction to form oligomers from coupling agent monomers is conducted. Subsequently, a two stage reaction, a polyurethane reaction and a radical polymerisation, is modelled based on an established approach. Using the final cured system, evaluations of averaged quantities during the reactions are carried out. Moreover, the system is evaluated along the normal direction of the fibre surface, which proves a spatial analysis of the fibre-sizing-resin interface.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.020
Threshold uncertainty score0.039

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0050.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.297
Teacher spread0.279 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2022
Admission routes2
Has abstractyes

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