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Record W4311719574 · doi:10.3390/molecules27248644

Research Progress on Graphite-Derived Materials for Electrocatalysis in Energy Conversion and Storage

2022· review· en· W4311719574 on OpenAlexafffund
Shuaijie He, Mingjie Wu, Li Song, Zhiyi Jiang, Hanlie Hong, Sylvain G. Cloutier, Huaming Yang, Sasha Omanovic, Shuhui Sun, Gaixia Zhang

Bibliographic record

VenueMolecules · 2022
Typereview
Languageen
FieldEnergy
TopicElectrocatalysts for Energy Conversion
Canadian institutionsÉcole de Technologie SupérieureMcGill UniversityInstitut National de la Recherche Scientifique
FundersFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of CanadaCentre québécois sur les matériaux fonctionnelsInstitut national de la recherche scientifiqueNational Natural Science Foundation of ChinaÉcole de technologie supérieureMcGill University
KeywordsElectrocatalystGraphiteGrapheneMaterials scienceElectrochemistrySurface modificationNanotechnologyOxygen evolutionElectrochemical energy conversionCarbon fibersFullereneHydrogen storageCarbon nanotubeChemical engineeringChemistryElectrodeOrganic chemistryComposite numberComposite materialPhysical chemistry

Abstract

fetched live from OpenAlex

High-performance electrocatalysts are critical to support emerging electrochemical energy storage and conversion technologies. Graphite-derived materials, including fullerenes, carbon nanotubes, and graphene, have been recognized as promising electrocatalysts and electrocatalyst supports for the oxygen reduction reaction (ORR), oxygen evolution reaction (OER), hydrogen evolution reaction (HER), and carbon dioxide reduction reaction (CO2RR). Effective modification/functionalization of graphite-derived materials can promote higher electrocatalytic activity, stability, and durability. In this review, the mechanisms and evaluation parameters for the above-outlined electrochemical reactions are introduced first. Then, we emphasize the preparation methods for graphite-derived materials and modification strategies. We further highlight the importance of the structural changes of modified graphite-derived materials on electrocatalytic activity and stability. Finally, future directions and perspectives towards new and better graphite-derived materials are presented.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.002
Threshold uncertainty score0.008

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0020.002
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0000.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.322
Teacher spread0.283 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations19
Published2022
Admission routes2
Has abstractyes

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