Vertical aligned solid‐state electrolyte templated by nanostructured “upright” cellulose film layers for advanced cell performance
Bibliographic record
Abstract
Abstract In this work, an “upright” cellulose layered template, which can be precisely controlled by the fiber orientation and thickness of anisotropic cellulose film, was first developed to prepare vertically aligned Li 7 La 3 Zr 2 O 12 (LLZO) ceramic membrane with low tortuosity and uniform porosity. The flexible composite solid‐state electrolytes (CSEs) were synthesized by incorporating poly(ethylene oxide) (PEO) polymer into LLZO architecture, and exhibited distinguished mechanical strength, elevated ionic conductivity (2.1 × 10 −4 S cm −1 ) and excellent interface compatibility with lithium anodes. The assembled LiFePO 4 /lithium full cells assembled with as‐obtained CSEs can reach large discharge capacities of 172.3 mAh g −1 with coulombic efficiencies of above 99% and capacity retention of 93.1% even after 200 cycles. These results clearly demonstrate that the sophisticated design of vertical aligned cellulose layered template with fine‐scale size and exquisite architecture is a promising and practical approach in fabricating flexible LLZO@PEO‐LiTFSI CSEs with high‐safety and high‐performance. image
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How this classification was reachedexpand
Full frame machine prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.
Distilled classifier scores by category (both heads)
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.001 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from itClassification
machine, unvalidatedMachine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.
How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".