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Record W4318020440 · doi:10.1016/j.recm.2023.01.001

Exploration of optimal reaction conditions on lactic acid production from glucose photoreforming over carbon nitride

2023· article· en· W4318020440 on OpenAlex
Heng Zhao, Xiao Wang, Xingxing Wu, Jiu Wang, Na Zhong, Ali Seifitokaldani, Steve Larter, Md Golam Kibria, Jinguang Hu

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueResources Chemicals and Materials · 2023
Typearticle
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsMcGill UniversityUniversity of Calgary
FundersFonds de recherche du Québec – Nature et technologiesAlliance de recherche numérique du CanadaCanada First Research Excellence FundNatural Sciences and Engineering Research Council of CanadaCanada Research Chairs
KeywordsLactic acidYield (engineering)Biomass (ecology)CatalysisCarbon nitrideChemistryGraphitic carbon nitrideChemical engineeringCarbon fibersMaterials sciencePhotocatalysisNanotechnologyOrganic chemistryBacteriaComposite materialBiology

Abstract

fetched live from OpenAlex

Biomass valorization by photoreforming approach provides a promising and alternative strategy to generate value-added chemicals and fuels. In this work, we demonstrate the selective production of lactic acid from glucose photoreforming over pristine graphitic carbon nitride (g-C3N4) photocatalyst. Control experiments screen the best condition for the highest yield of lactic acid, including modulating pH, catalyst loading, and reaction time. 100% glucose conversion is achieved along with almost 100% lactic acid yield under the optimized condition. Density functional theory (DFT) calculations reveal that the rate-determining step (RDS) of the overall reaction on g-C3N4 is the conversion of pyruvaldehyde, where an electron transfer takes place. This present work provides experimental insights and theoretical understanding for selective lactic acid production from biomass photoreforming.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.531

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.278
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it