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Record W4318194845 · doi:10.1002/cjce.24859

Recent advances in hydrogen production through catalytic steam reforming of ethanol: Advances in catalytic design

2023· article· en· W4318194845 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
venuePublished in a venue whose home country is Canada.

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2023
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsUniversity of Regina
FundersNatural Sciences and Engineering Research Council of CanadaMitacsCanada Foundation for InnovationUniversity of Regina
KeywordsSteam reformingCatalysisBimetallic stripHydrogen productionChemical engineeringSelectivityHydrogenMaterials scienceCatalyst supportChemistryInorganic chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Catalytic reforming is a promising technology for producing renewable fuels; however, developing highly stable, efficient, green, and economical metallic catalysts that reduce metal sintering and carbon formation while improving catalyst activity, selectivity, and stability remains a major issue. In this regard, numerous studies have been documented in the past couple of decades evaluating the effects of various supports and promoters using ethanol as a co‐reactant in the catalytic steam reforming to produce energy‐efficient gaseous fuel, that is, hydrogen. This review article compiles research work focused on the catalytic reforming of ethanol reported in the last decade. Also, the outcomes of experimental studies have been presented and discussed for parametric analysis as case studies. The review shows that ethanol conversion, hydrogen selectivity, and catalyst stability are strongly influenced by the physicochemical properties of the catalyst, synthesis method, support choice, promoters, temperature, pressure, steam‐to‐ethanol ratio, and hourly space velocity. Noble metals (e.g., Pt, Rh, Ru, Pd, and Au), transition metals (e.g., Ni, Co, and Cu), and bimetallic composites were the most used catalysts in ethanol‐steam reforming reactions. Also, proper selection of support and promoter plays a significant role in modifying catalyst morphology, surface area, and particle size, enhancing selectivity, and reducing catalyst carbon deposition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.516
Threshold uncertainty score0.803

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.002
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.244
Teacher spread0.225 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it