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Record W4318987249 · doi:10.1002/aelm.202200910

Synthesis and Characterization of a New Ferroelectric with Low Lead Content, a High Curie Temperature, and a High Piezoelectric Response

2023· article· en· W4318987249 on OpenAlexafffund
Thomas Rowe, Brooke N. Richtik, Michelle Dolgos

Bibliographic record

VenueAdvanced Electronic Materials · 2023
Typearticle
Languageen
FieldMaterials Science
TopicFerroelectric and Piezoelectric Materials
Canadian institutionsUniversity of Calgary
FundersArgonne National LaboratoryOffice of ScienceCanada First Research Excellence FundU.S. Department of Energy
KeywordsCurie temperatureMaterials scienceFerroelectricityPhase boundaryPiezoelectricityPolarization (electrochemistry)Analytical Chemistry (journal)DopingAtmospheric temperature rangeCondensed matter physicsHysteresisCuriePhase (matter)OptoelectronicsComposite materialThermodynamicsDielectricPhysical chemistryFerromagnetismChemistryPhysics

Abstract

fetched live from OpenAlex

Abstract A new solid solution (1−x)Bi(Fe2/8Ti3/8Mg3/8)O3–(x)PbTiO3 (BFTM‐PT) is synthesized and the electromechanical properties are measured. This system is defined as a low‐lead material with ferroelectric/piezoelectric behavior and a morphotropic phase boundary (MPB) that leads to enhanced properties. The MPB is located between x = 0.30 and 0.35 and coincides with a structural phase transition and a sharp increase in the piezoelectric response. The system demonstrates ferroelectric hysteresis where x = 0.325 displays the best properties with a maximum polarization of 39 µC cm−2 and a remnant polarization of 26 µC cm−2. The range of compositions has high Curie temperature (Tc), ranging from 625–650 °C. Materials with a Tc above 400 °C typically have a low d33 of <50 pC N−1 at room temperature. However, BFTM‐PT has a higher d33 that most other compositions with a Tc in this range, with the highest being 145 pC N−1 for x = 0.375. The d33 drops off above 100 °C, but doping studies can be done in the future to stabilize the piezoelectric response at higher temperatures. These outstanding properties open the possibility of new transducer applications, in particular ones requiring high temperature and high power.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.221
Teacher spread0.212 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2023
Admission routes2
Has abstractyes

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