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Record W4319862280 · doi:10.1002/cjce.24835

Degradation study of some pharmaceuticals in commercial formulation by <scp>electro‐Fenton</scp> process using a dimensionally stable anode cathode: Analytical technique, optimization conditions, and energy consumption

2023· article· en· W4319862280 on OpenAlexvenueno aff
Foffié Thiery Auguste Appia, Lassiné Ouattara

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicAdvanced oxidation water treatment
Canadian institutionsnot available
Fundersnot available
KeywordsCathodeAnodeDegradation (telecommunications)ElectrochemistryKineticsChemistryWastewaterElectrodeEnergy consumptionNuclear chemistryAnalytical Chemistry (journal)Materials scienceChromatographyEnvironmental engineeringComputer sciencePhysicsPhysical chemistryElectrical engineeringEnvironmental science

Abstract

fetched live from OpenAlex

Abstract The aim of this work was to degrade pharmaceuticals such as amoxicillin (AMX), ceftriaxone (CTX), and Telebrix (TLX) by electro‐Fenton (EF) process using a dimensionally stable anode (DSA) cathode, Pt‐RuO 2 ‐IrO 2 (PRI). For this purpose, the optimal conditions of degradation, the pseudo‐first‐order kinetics, the current efficiency, the electrochemical energy consumption (EEC), and the energy cost have been investigated. A spectrophotometric analysis technique has been developed. It is a simple, fast, linear, reliable, and selective technique with LOD = 0.013 g/L and LOQ = 0.04 g/L. The optimum working conditions determined are: Fe 2+ = 0.2 mM, pH = 3, j = 20 mA/cm 2 , and (Pt, PRI) as electrode pair. Under these conditions, the EF process leads to a conversion of the parent compound. In addition, the degradation of compounds by EF follows pseudo‐first‐order kinetics. The EEC for the degradation of 1 kg COD of an organic compound is 99.48, 66.86, and 50.32 kWh kg COD −1 for AMX, CTX, and TLX respectively. The energy cost for processing these compounds is $4.92 (AMX), $10.03 (CTX), and $7.55 (TLX) with current efficiencies between 26% and 51%. Ultimately, the EF process using PRI at the cathode can be used for the treatment of real wastewater from health centres under optimal conditions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.033
Threshold uncertainty score0.337

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.020
GPT teacher head0.279
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2023
Admission routes1
Has abstractyes

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