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Record W4323835878 · doi:10.1103/physrevb.107.l100501

Superconductivity in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Li</mml:mi><mml:mn>8</mml:mn></mml:msub><mml:mi>Au</mml:mi></mml:mrow></mml:math> electride

2023· article· lv· W4323835878 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenuePhysical review. B./Physical review. B · 2023
Typearticle
Languagelv
FieldChemical Engineering
TopicAmmonia Synthesis and Nitrogen Reduction
Canadian institutionsUniversity of Saskatchewan
FundersNational Key Research and Development Program of ChinaPostdoctoral Science Foundation of Jiangsu ProvinceNatural Sciences and Engineering Research Council of CanadaMinisterio de Ciencia e InnovaciónEusko JaurlaritzaNatural Science Foundation of Hebei ProvinceNational Natural Science Foundation of ChinaDepartment of Education of Hebei ProvinceEuskal Herriko Unibertsitatea
KeywordsPhysicsSuperconductivityCoupling (piping)CrystallographyIonLattice vibrationCondensed matter physicsMaterials scienceAtomic physicsPhononChemistryQuantum mechanics

Abstract

fetched live from OpenAlex

Located at crystal voids, interstitial anion electrons (IAEs) have diverse topologies, which may be tuned to achieve different properties. Elucidating the role of IAEs in electron-phonon coupling (EPC), and using it to design electride superconductors, leads to the current prediction of superconducting ${\mathrm{Li}}_{8}\mathrm{Au}$ at high pressure. We suggest that the occurence of high-temperature superconductivity in electrides requires high-symmetry structures with hydrogenlike cages, an electron acceptor element to balance charges, and isolated IAEs coupled with medium-frequency vibrations. The uniquely designed ${\mathrm{Li}}_{8}\mathrm{Au}$ electride has a NaCl-type ($B1$) lattice, with atomic Au and cubic ${\mathrm{Li}}_{8}$ cages as bases. Isolated IAEs are formed at the cage centers, with extra charges taken up by Au. These octahedrally coordinated IAEs have a $p$-orbital-like attribute and are strongly coupled with atomic vibrations in the ${\mathrm{Li}}_{8}$ cages. The strong EPC in ${\mathrm{Li}}_{8}\mathrm{Au}$ results in a calculated ${T}_{c}$ of 73.1 K at 250 GPa, which is the highest ${T}_{c}$ reported to date for all the electrides. A slight substitutional Pt doping can enhance the ${T}_{c}$ of ${\mathrm{Li}}_{8}\mathrm{Au}$ to exceed liquid nitrogen temperature.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.004
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.895
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.004
Meta-epidemiology (narrow)0.0010.002
Meta-epidemiology (broad)0.0010.003
Bibliometrics0.0000.003
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0010.003
Insufficient payload (model declined to judge)0.0520.007

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.281
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it