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Record W4323835878 · doi:10.1103/physrevb.107.l100501

Superconductivity in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mrow><mml:msub><mml:mi>Li</mml:mi><mml:mn>8</mml:mn></mml:msub><mml:mi>Au</mml:mi></mml:mrow></mml:math> electride

2023· article· lv· W4323835878 on OpenAlexafffund
Xiaohua Zhang, Yansun Yao, Shicong Ding, Aitor Bergara, Fei Li, Yong Liu, Xiang‐Feng Zhou, Guochun Yang

Bibliographic record

VenuePhysical review. B./Physical review. B · 2023
Typearticle
Languagelv
FieldChemical Engineering
TopicAmmonia Synthesis and Nitrogen Reduction
Canadian institutionsUniversity of Saskatchewan
FundersNational Key Research and Development Program of ChinaPostdoctoral Science Foundation of Jiangsu ProvinceNatural Sciences and Engineering Research Council of CanadaMinisterio de Ciencia e InnovaciónEusko JaurlaritzaNatural Science Foundation of Hebei ProvinceNational Natural Science Foundation of ChinaDepartment of Education of Hebei ProvinceEuskal Herriko Unibertsitatea
KeywordsPhysicsSuperconductivityCoupling (piping)CrystallographyIonLattice vibrationCondensed matter physicsMaterials scienceAtomic physicsPhononChemistryQuantum mechanics

Abstract

fetched live from OpenAlex

Located at crystal voids, interstitial anion electrons (IAEs) have diverse topologies, which may be tuned to achieve different properties. Elucidating the role of IAEs in electron-phonon coupling (EPC), and using it to design electride superconductors, leads to the current prediction of superconducting ${\mathrm{Li}}_{8}\mathrm{Au}$ at high pressure. We suggest that the occurence of high-temperature superconductivity in electrides requires high-symmetry structures with hydrogenlike cages, an electron acceptor element to balance charges, and isolated IAEs coupled with medium-frequency vibrations. The uniquely designed ${\mathrm{Li}}_{8}\mathrm{Au}$ electride has a NaCl-type ($B1$) lattice, with atomic Au and cubic ${\mathrm{Li}}_{8}$ cages as bases. Isolated IAEs are formed at the cage centers, with extra charges taken up by Au. These octahedrally coordinated IAEs have a $p$-orbital-like attribute and are strongly coupled with atomic vibrations in the ${\mathrm{Li}}_{8}$ cages. The strong EPC in ${\mathrm{Li}}_{8}\mathrm{Au}$ results in a calculated ${T}_{c}$ of 73.1 K at 250 GPa, which is the highest ${T}_{c}$ reported to date for all the electrides. A slight substitutional Pt doping can enhance the ${T}_{c}$ of ${\mathrm{Li}}_{8}\mathrm{Au}$ to exceed liquid nitrogen temperature.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.015

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0050.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.281
Teacher spread0.259 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations67
Published2023
Admission routes2
Has abstractyes

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