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Record W4323926008 · doi:10.1021/acsphotonics.2c01968

Ultrafast Heat Transfer at the Nanoscale: Controlling Heat Anisotropy

2023· article· en· W4323926008 on OpenAlexafffund
Jean‐François Bryche, Marlo Vega, Julien Moreau, Paul‐Ludovic Karsenti, Paul Bresson, Mondher Besbes, Philippe Gogol, Denis Morris, Paul G. Charette, Michael Canva

Bibliographic record

VenueACS Photonics · 2023
Typearticle
Languageen
FieldMaterials Science
TopicGold and Silver Nanoparticles Synthesis and Applications
Canadian institutionsInstitut interdisciplinaire d'innovation technologiqueUniversité de Sherbrooke
FundersÉcole Centrale de LyonInstitut National des Sciences Appliquées de LyonNatural Sciences and Engineering Research Council of CanadaUniversité de SherbrookeUniversité Paris-SaclayCentre National de la Recherche ScientifiqueFonds de recherche du Québec – Nature et technologiesUniversité Grenoble AlpesAgence Nationale de la Recherche
KeywordsMaterials scienceUltrashort pulseFemtosecondHeat transferNanostructureNanoscopic scalePhotothermal therapyHeat generationOptoelectronicsPlasmonAnisotropyUltrafast laser spectroscopyNanoparticleOpticsNanotechnologyMechanicsLaserPhysicsThermodynamics

Abstract

fetched live from OpenAlex

Thermoplasmonics has benefited from increasing attention in recent years by exploiting the photothermal effects within plasmonic nanoparticles to generate nanoscale heat sources. Recently, it has been demonstrated that exciting gold nanoparticles with ultrashort light pulses could be used to achieve high-speed light management and nanoscale heat-sensitive chemical reaction control. In this work, we study non-uniform thermal energy transient distribution inside cross-shaped nanostructures with femtosecond transient spectroscopy coupled to a thermo-optical numerical model, free of fitting parameters. We show experimentally and numerically that the polarization of the excitation light can control the heat distribution in the nanostructures. We also demonstrate the necessity of considering nonthermal electron ballistic displacement in fast transient heat dynamics models.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.025
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.238
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2023
Admission routes2
Has abstractyes

Explore more

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