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Record W4327545669 · doi:10.1016/j.optmat.2023.113648

Growth, structure refinement, thermal expansion and optical spectroscopy of Tm3+-doped MgMoO4

2023· article· en· W4327545669 on OpenAlexfundno aff
К. А. Субботин, Anatolii I. Titov, D. A. Lis, Yulia I. Zimina, Y.S. Didenko, Ghassen Zin Elabedine, Kirill Eremeev, Rosa Maria Solé, Magdalena Aguiló, Pavel A. Volkov, П. А. Попов, E. V. Chernova, Francesc Dı́az, Patrice Camy, Pavel Loiko, Xavier Mateos

Bibliographic record

VenueOptical Materials · 2023
Typearticle
Languageen
FieldEngineering
TopicSolid State Laser Technologies
Canadian institutionsnot available
FundersAgencia Estatal de InvestigaciónEuropean Regional Development FundNational Research Council CanadaMinistry of Science and Higher Education of the Russian FederationMinisterio de Ciencia e InnovaciónMinisterstwo Edukacji i NaukiMinistry of Education and Science of the Russian Federation
KeywordsThuliumMonoclinic crystal systemMolybdateSpectroscopyRaman spectroscopyDopingAnalytical Chemistry (journal)Excited stateThermal expansionIonNegative thermal expansionLaserChemistryMaterials scienceCrystal structureOpticsCrystallographyAtomic physicsOptoelectronicsInorganic chemistry

Abstract

fetched live from OpenAlex

Thulium-doped magnesium molybdate single-crystal (Tm3+:MgMoO4) was grown by the Czochralski method (melting point: 1322 °C). The actual Tm3+ doping level was measured to be 0.1 at.% (the segregation coefficient was only 0.02). Tm:MgMoO4 belongs to the monoclinic class (sp. gr. C2/m, lattice constants: a = 10.2769(2) Å, b = 9.2898(5) Å, c = 7.0269(4) Å, β = 106.898(6)°). The thermal expansion tensor of this crystal is determined. Its thermal conductivity is also measured at 50–300 K (at room temperature, it amounts to 2.64 Wm−1K−1). Polarized Raman spectra are presented and the strongest mode is found at 957 cm−1. Optical spectroscopy of Tm3+ ions is studied indicating broad emission bands extending beyond 2 μm (the 3F4 → 3H6 transition) and a long lifetime of the 3F4 excited-state (1.972 ms). This makes Tm:MgMoO4 promising for broadly tunable and mode-locked lasers, when the technological problem of fabricating crystals with higher Tm3+ concentrations will be solved.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.013

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.233
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2023
Admission routes1
Has abstractyes

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