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Record W4327572165 · doi:10.1021/acsenergylett.3c00242

Electrochemical Cement Clinker Precursor Production at Low Voltages

2023· article· en· W4327572165 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Energy Letters · 2023
Typearticle
Languageen
FieldMaterials Science
TopicAdvancements in Solid Oxide Fuel Cells
Canadian institutionsCanadian Institute for Advanced ResearchUniversity of British Columbia
FundersCanada Foundation for InnovationNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanadian Institute for Advanced Research
KeywordsCementKilnElectrolysisClinker (cement)Materials scienceWaste managementElectrochemistryFossil fuelEnvironmental scienceOxidizing agentMetallurgyElectrodeChemistryEngineering

Abstract

fetched live from OpenAlex

Cement production is carbon intensive today because fossil fuels are used to heat high-temperature kilns, and because CO 2 is released as a byproduct of limestone (CaCO 3 ) decomposition. Electrochemical reactors can decarbonize cement production by using electricity instead of heat to convert CaCO 3 into Ca(OH) 2, a cement clinker precusor, while releasing the CO 2 byproduct as a pure stream. Herein, we report a “cement electrolyzer” that electrolytically converts limestone into Ca(OH) 2 at a cell voltage of 1.8 V at 100 mA cm –2 . This new benchmark improves upon the previous record of 4.2 V by oxidizing the H 2 byproduct from the cathode compartment into protons for CaCO 3 decomposition. A techno-economic model shows that this use of H 2 decreases the cost of cement production by $36/t cement compared to the use of H 2 as a kiln fuel. This work describes an energy-efficient cement electrolyzer and advances the feasibility of electrochemical cement production.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.016
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.246
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it