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Record W4327951425 · doi:10.5194/acp-23-3493-2023

Estimating enhancement ratios of nitrogen dioxide, carbon monoxide and carbon dioxide using satellite observations

2023· article· en· W4327951425 on OpenAlexafffund
Cameron G. MacDonald, Jon‐Paul Mastrogiacomo, Joshua L. Laughner, Jacob K. Hedelius, Ray Nassar, Debra Wunch

Bibliographic record

VenueAtmospheric chemistry and physics · 2023
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsEnvironment and Climate Change CanadaUniversity of TorontoUniversity of Waterloo
FundersCanadian Space Agency
KeywordsEnvironmental scienceCarbon dioxideMegacityNitrogen dioxideAtmospheric sciencesGreenhouse gasTroposphereSatelliteCarbon monoxidePopulationObservatoryMeteorologyClimatologyChemistryGeographyGeologyPhysicsOceanography

Abstract

fetched live from OpenAlex

Using co-located space-based measurements of carbon dioxide (CO 2 ) from the Orbiting Carbon Observatory-2 and Orbiting Carbon Observatory-3 (OCO-2/3) and carbon monoxide (CO) and nitrogen dioxide (NO 2 ) from the TROPOspheric Monitoring Instrument (TROPOMI), we calculate total column enhancements for observations influenced by anthropogenic emissions from urban regions relative to clean background values. We apply this method to observations taken over or downwind of 27 large (population of >1 million) urban areas from around the world. Enhancement ratios between species are calculated and compared to emissions ratios derived from four globally gridded anthropogenic emissions inventories. We find that these global inventories underestimate CO emissions in many North American and European cities relative to our observed enhancement ratios, while smaller differences were found for NO 2 emissions. We further demonstrate that the calculation and intercomparison of enhancement ratios of multiple tracers can help to identify the underlying biases leading to disagreement between observations and inventories. Additionally, we use high-resolution CO 2 inventories for two cities (Los Angeles and Indianapolis) to estimate emissions of CO and NO 2 using our calculated enhancement ratios and find good agreement with both a previous modelling study for the megacity of Los Angeles and California Air Resources Board (CARB) inventory estimates.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.015
Threshold uncertainty score0.030

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.214
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations36
Published2023
Admission routes2
Has abstractyes

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