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Record W4361207168 · doi:10.1021/acs.iecr.2c04125

Ultrahigh Electromagnetic Wave Transmitting Polyphenylene Sulfide Microcellular Foams Based on Molecular Structure Design for 5G Communication

2023· article· en· W4361207168 on OpenAlexaff
Lisha Zhang, Dengyang Chen, Bihui Jin, Bowen Zhang, Pengjian Gong, Bing Zhang, Chul B. Park, Guangxian Li

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2023
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Foaming and Composites
Canadian institutionsUniversity of Toronto
FundersState Key Laboratory of Polymer Materials EngineeringMinistry of Education of the People's Republic of ChinaNational Natural Science Foundation of ChinaInternational S and T Cooperation Program of Sichuan Province
KeywordsMaterials scienceDielectricComposite materialDielectric lossNucleationTransmission lossOptoelectronicsOpticsOrganic chemistry

Abstract

fetched live from OpenAlex

In the scenario of fifth-generation communication, especially millimeter wave (mmW) transmission, microelectronic material is required to have better signal stability, that is, a lower dielectric constant ( D k ) and dielectric loss ( D f ). This work takes full advantage of the low dielectric molecular structure characteristics in polyphenylene sulfide (PPS) and the nonresidual low dielectric characteristics of supercritical CO 2 (scCO 2 ) foaming to enhance the low dielectric performance. The distinct structure of a highly stable thioether bond and highly reactive hydrogen in the benzene ring in the PPS macromolecule enables the oxo-bridging between PPS molecular chains and hence increases PPS melt strength. By further adjusting the regularity in PPS molecular chains to broaden the melting range of PPS crystals, the PPS microcellular foam of large expansion ratio (16.5-fold) with uniform cells is obtained. It has an ultralow D k of 1.14 and D f of 0.0005 at 3 GHz. In the Ka band of 26–40 GHz, the broadband signal transmission has nearly no loss (∼99%). Furthermore, it has a low density (<0.08 g/cm 3 ), is hydrophobic (contact angle of 123.4°), and reaches V-0 level flame retardancy. This ultrahigh mmW transmission material with excellent comprehensive performance provides an alternative for solving the problems of mmW propagation in the existing dielectric materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.040
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.063
GPT teacher head0.289
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations28
Published2023
Admission routes1
Has abstractyes

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