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Record W4362697629 · doi:10.1021/acsaom.3c00019

Flexible Composite Inverse Opal Fabrics for Visual Detection of BTEX Vapor

2023· article· en· W4362697629 on OpenAlexaff
Xinbo Gong, Chengyi Hou, Qinghong Zhang, Yaogang Li, Hongzhi Wang, Michael J. Serpe

Bibliographic record

VenueACS Applied Optical Materials · 2023
Typearticle
Languageen
FieldPhysics and Astronomy
TopicPhotonic Crystals and Applications
Canadian institutionsUniversity of Alberta
FundersShanghai Rising-Star ProgramCentral University Basic Research Fund of ChinaDonghua UniversityNational Natural Science Foundation of China
KeywordsMaterials scienceCoatingNanotechnologyPhotonic crystalChemical engineeringComposite materialOptoelectronics

Abstract

fetched live from OpenAlex

Photonic crystal (PC) is widely used in BTEX vapor colorimetric detection due to its tunable photonic band gap, which has battery-free and signal output instrument-free advantages. Recently, responsive PC fabrics have also attracted a lot of interest. Compared to hard substrates such as glass slide and silicon wafer, these fabrics have better flexibility and portability, which can make them more widely usable. However, at present, the PC fabrics are mainly achieved by deposition of colloidal microspheres or nanosheets, which are easy to be destroyed by stretching, bending, and washing, and the dense stacked structure hinder the diffusion of vapor as well. In this study, the PEGDA inverse opal structure (IOs) with a porous structure and an ultrahigh specific area was constructed on polyester fabrics by sacrificing SiO 2 PC template of glass/SiO 2 PCs/fabric sandwich structure, and the IOs coating showed a very good bonding force with the fabrics. Benefiting from the porous structure of IOs coating, the diffusion rate of vapor was greatly increased. Besides, functional polymers and flexible MOFs were infiltrated into the IOs to selectively absorb BTEX and enhance the absorption as well, thus effectively reducing the detection limits (2.92, 1.85, 0.52, and 0.13 g/m 3 for benzene, toluene, ethylbenzene, xylene, respectively) and response speed (0.3 s for response and 0.8 s for recover), and in addition, the repeatability was good after 10 cycles. More importantly, the method to construct IOs on fabrics was universal; the IOs can be replaced with any polymer, so it is expected to be applied for the detection of other analytes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.060
Threshold uncertainty score0.501

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.281
Teacher spread0.264 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2023
Admission routes1
Has abstractyes

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