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Crucial role of Ce particles during initial hydrogen absorption of AB-type hydrogen storage alloys

2023· article· en· 60 citations· W4367301476 on OpenAlex· 10.1016/j.nanoen.2023.108483

Why is this work in the frame?

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

Canadian funderA Canadian agency funded it. The work may carry no Canadian affiliation at all.

No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Full frame distilled prediction

Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

Candidate categories
none
Consensus categories
none
Domain
Candidate signal: noneConsensus signal: none
Study design
Candidate signal: Bench or experimentalConsensus signal: Bench or experimental
Genre
Candidate signal: EmpiricalConsensus signal: Empirical
Teacher disagreement score
0.005
Threshold uncertainty score
0.724
Validation status
machine_predicted_unvalidated · codex-gemma-dda1882f352a

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Opus teacher head0.015
GPT teacher head0.248
Teacher spread
0.233 · how far apart the two teachers sit on this one work
Validation status
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Abstract

The hydrogen storage behavior and the microstructural features of AB-type Ti50Fe48V2 hydrogen storage alloys containing a small amount of cerium (Ce) were investigated to understand the effect of Ce addition during initial hydrogen absorption. The initial hydrogen absorption kinetics of the alloys improved significantly at room temperature with Ce addition, which exhibited no significant influence on the pressure-composition isotherms for hydrogen absorption and desorption. Fine spherical particles containing Ce, which were determined to be γ-Ce mixed with cerium oxide, were dispersed in the ordered body-centered cubic TiFe matrix. During the early stage of hydrogen absorption, small cracks were initiated around the Ce particles, likely caused by the volume expansion owing to the formation of ε-CeH2. Subsequently, many large cracks, believed to have formed owing to the hydrogenation of the TiFe matrix, propagated during further hydrogen absorption. Therefore, these Ce particles appear to play a crucial role by providing starting points for the initial hydrogenation, with this mechanism explaining the significant increase in the primary hydrogen absorption kinetics after Ce addition. Notably, some small pits were observed after partial hydrogen absorption, possibly attributed to the hydrogenation of Ce particles underneath the alloy surfaces.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

The record

Venue
Nano Energy
Topic
Hydrogen Storage and Materials
Field
Materials Science
Canadian institutions
not available
Funders
Korea Institute of Science and TechnologyMinistry of Trade, Industry and EnergyNational Research Foundation of KoreaMinistry of EducationCHEO Research Institute
Keywords
Materials scienceHydrogen storageHydrogenCeriumAlloyAbsorption (acoustics)KineticsDesorptionChemical engineeringInorganic chemistryMetallurgyComposite materialPhysical chemistryChemistryOrganic chemistryAdsorption
Has abstract in OpenAlex
yes