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Record W4367309171 · doi:10.1016/j.mtadv.2023.100373

Wafer-scale Ge freestanding membranes for lightweight and flexible optoelectronics

2023· article· en· W4367309171 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueMaterials Today Advances · 2023
Typearticle
Languageen
FieldMaterials Science
TopicSilicon Nanostructures and Photoluminescence
Canadian institutionsInstitut interdisciplinaire d'innovation technologiqueUniversité de Sherbrooke
FundersInstitut National des Sciences Appliquées de LyonCentre National de la Recherche ScientifiqueFonds de recherche du Québec – Nature et technologiesUmicoreUniversité Grenoble AlpesNatural Sciences and Engineering Research Council of CanadaFonds de recherche du QuébecUniversité de SherbrookeMitacsIndian National Science Academy
KeywordsMaterials scienceWaferEpitaxySurface roughnessNucleationCoalescence (physics)Substrate (aquarium)NanotechnologySurface finishNanoscopic scaleOptoelectronicsPorosityComposite materialLayer (electronics)Chemistry

Abstract

fetched live from OpenAlex

Semiconductor-based freestanding membranes (FSM) have recently emerged as a highly promising area of advanced materials research. Their unique properties, such as lightweight and flexibility, make them attractive for a wide range of disruptive device applications. However, the production of high-quality, single-crystalline FSM, especially from elemental materials such as germanium (Ge), remains a significant challenge. In this work, we report on the formation of easily detachable wafer-scale Ge FSM on porous Ge (PGe) substrate. The proposed method relies on low-temperature Ge epitaxy, allowing to preserve the porous structure's integrity during the FSM formation, and an easy substrate preparation for multiple reuses. Analysis of the surface morphology as a function of the deposited Ge thickness reveals that the FSM formation occurs in two distinct regimes. During the initial epitaxial regime, the Ge growth is governed by 3D nucleation on the PGe top surface. The nanoscale islands size increase, and consequent coalescence are found to increase the surface roughness up to a critical thickness, allowing full coalescence of islands into a 2D epilayer. The analysis of the membrane's surface morphology for various thicknesses shows continuous improvement, achieving sub nanometer surface roughness. Moreover, we demonstrate that the FSM formation process is applicable regardless the PGe porosity and thickness, while offering facile and sustainable substrate reconditioning for multiple FSM generation from the same substrate. Our findings open new opportunities to produce lightweight and flexible, high-performance optoelectronics based on Ge FSM, while ensuring reduction of both cost and critical materials consumption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.054
Threshold uncertainty score0.772

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.264
Teacher spread0.253 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it