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Record W4367315930 · doi:10.1002/marc.202300162

A Novel Anderson‐Type POMs‐Based Hybrids Flame Retardant for Reducing Smoke Release and Toxicity of Epoxy Resins

2023· article· en· W4367315930 on OpenAlexaff
Hui Xu, Chaohua Peng, Long Xia, Zhongxi Miao, Siyuan He, Cheng Chi, Weiang Luo, Guorong Chen, Birong Zeng, Shuchuan Wang, Lizong Dai

Bibliographic record

VenueMacromolecular Rapid Communications · 2023
Typearticle
Languageen
FieldChemical Engineering
TopicCarbon dioxide utilization in catalysis
Canadian institutionsNovelis (Canada)
FundersNational Natural Science Foundation of China
KeywordsFire retardantSmokeEpoxyMaterials scienceCarbonizationComposite materialNuclear chemistryChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Smoke emission and smoke toxicity have drawn more attention to improving the fire safety of polymers. In this work, a polyoxometalates (POMs)‐based hybrids flame retardant (P‐AlMo 6 ) epoxy resin (EP) is prepared with toxicity‐reduction and smoke‐suppression properties via a peptide coupling reaction between POMs and organic molecules with double DOPO (bisDOPA). It combines the good compatibility of the organic molecule and the superior catalytic performance of POMs. Compared to pure EP, the glass transition temperature and flexural modulus of EP composite with 5 wt.% P‐AlMo 6 (EP/P‐AlMo 6 ‐5) are raised by 12.3 °C and 57.75%, respectively. Notably, at low flame‐retardant addition, the average CO to CO 2 ratio (Av‐COY/Av‐CO 2 Y) is reduced by 33.75%. Total heat release (THR) and total smoke production (TSP) are lowered by 44.4% and 53.7%, respectively. The Limited Oxygen Index (LOI) value achieved 31.7% and obtained UL‐94 V‐0 rating. SEM, Raman, X‐ray photoelectron spectroscopy, and TG‐FTIR are applied to analyze the flame‐retardant mechanism in condensed and gas phase. Outstanding flame retardant, low smoke toxicity properties are attained due to the catalytic carbonization ability of metal oxides Al 2 O 3 and MoO 3 produced from the breakdown of POMs. This work advances the development of POMs‐based hybrids flame retardants with low smoke toxicity properties.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.450
Threshold uncertainty score0.922

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.049
GPT teacher head0.293
Teacher spread0.244 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2023
Admission routes1
Has abstractyes

Explore more

Same venueMacromolecular Rapid CommunicationsSame topicCarbon dioxide utilization in catalysisFrench-language works237,207