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Record W4367693978 · doi:10.1016/j.susmat.2023.e00627

Estimation of life cycle greenhouse gas emissions of asphaltene-based carbon fibers derived from oil sands bitumen

2023· article· en· W4367693978 on OpenAlexafffund
Miguel Baritto, A.O. Oni, Amit Kumar

Bibliographic record

VenueSustainable materials and technologies · 2023
Typearticle
Languageen
FieldEngineering
TopicFiber-reinforced polymer composites
Canadian institutionsUniversity of Alberta
FundersAlberta InnovatesUniversity of Alberta
KeywordsGreenhouse gasAsphaltLife-cycle assessmentAsphalteneEnvironmental scienceFossil fuelCarbon footprintCarbon fibersRaw materialPulp and paper industryWaste managementEnvironmental engineeringMaterials scienceProduction (economics)ChemistryEngineeringComposite materialOrganic chemistryGeology

Abstract

fetched live from OpenAlex

Bitumen-derived asphaltenes have emerged as a potential precursor for carbon fiber production. The technology to make it possible is in the early stages of research and development and so there are no studies on the GHG emissions from the process, which are critical to compare its carbon footprint with that of polyacrylonitrile (PAN), the standard precursor for carbon fiber production. The asphaltene-based carbon fiber (ACF) life cycle stages are bitumen production, asphaltene separation, precursor manufacturing, and carbon fiber production. In this study, we developed data-intensive models to estimate the life cycle GHG emissions of ACF. Sensitivity and uncertainty analyses were also performed to determine the inputs that have the largest effect on the GHG emissions of ACF. The results show that the life cycle GHG emissions of ACF are 16.2 kg CO2eq/kg CF. This value represents a reduction of 68.7% compared to PAN-based carbon fiber. The carbon fiber production stage is the most emission-intensive, mainly because of the high consumption of electricity. When uncertainty is considered, the life cycle GHG emissions of ACF range from 10.4 to 21.8 kg CO2eq/kg CF. The outcome of this study confirms the potential of asphaltenes as a low-carbon intense raw material for carbon fiber production.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score0.068

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.196
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2023
Admission routes2
Has abstractyes

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