MétaCan
Menu
Back to cohort
Record W4375865554 · doi:10.1002/jrs.6541

Raman spectroscopic study of the transformation of nitrogen‐bearing K‐cymrite during heating experiments: Origin of kokchetavite in high‐pressure metamorphic rocks

2023· article· en· W4375865554 on OpenAlexaff
Andrey V. Korsakov, Alexandr V. Romanenko, Alexander G. Sokol, Kira Musiyachenko

Bibliographic record

VenueJournal of Raman Spectroscopy · 2023
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeological and Geochemical Analysis
Canadian institutionsUniversity of British Columbia
FundersRussian Science Foundation
KeywordsNitrogenRaman spectroscopyMetamorphic rockMantle (geology)GeologySubductionAnalytical Chemistry (journal)AnhydrousMineralogyMaterials scienceGeochemistryChemistryTectonics

Abstract

fetched live from OpenAlex

Abstract Nitrogen‐bearing K‐cymrite was synthesized in experiments at high pressures but so far has not been found/identified as inclusions in minerals subducted and subsequently exhumed from mantle depths. K‐cymrite is a potential carrier of nitrogen; it can store and transport up to 4 wt% of nitrogen in the deep mantle, thus contributing to the global nitrogen cycle. The stability of nitrogen‐bearing K‐cymrite synthesized at pressure of 6.3 GPa, upon exhumation to the Earth's surface, remains unknown. Here, we report an in situ Raman spectroscopic study of nitrogen‐bearing K‐cymrite, using Linkam heating and freezing microscope stage (THMS600). The transition induced in this experiment corresponds to the retrograde PT‐path of deeply subducted rocks. Our results demonstrate that (i) nitrogen‐bearing K‐cymrite structure is more stable upon heating than pure H2O bearing specimens (KAlSi3O8·H2O), (ii) phase transformation (e.g., H2O, N2, and NH3 release) starts at 550°C leading to the formation of kokchetavite (an anhydrous hexagonal polymorph of KAlSi3O8) frequently observed in high‐pressure metamorphic rocks, and (iii) Raman spectra of kokchetavite obtained from different precursors (e.g., nitrogen‐bearing and H2O‐bearing K‐cymrite) are identical. Thus, nitrogen‐bearing K‐cymrite can be considered a potential host phase for nitrogen in subduction‐related environments, and it can be preserved as inclusions in refractory minerals during the exhumation of deeply subducted rocks.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.248
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2023
Admission routes1
Has abstractyes

Explore more

Same venueJournal of Raman SpectroscopySame topicGeological and Geochemical AnalysisFrench-language works237,207