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Record W4376254854 · doi:10.26434/chemrxiv-2023-0zcw9

Electrolytic cement clinker production sustained through orthogonalization of ion vectors

2023· preprint· en· W4376254854 on OpenAlex
Zishuai Zhang, Benjamin A. W. Mowbray, Colin Parkyn, Yongwook Kim, Curtis P. Berlinguette

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueChemRxiv · 2023
Typepreprint
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsCanadian Institute for Advanced ResearchUniversity of British Columbia
FundersCanada First Research Excellence FundNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsCanadian Institute for Advanced Research
KeywordsElectrolysisCementMaterials scienceChemical engineeringElectrochemistryClinker (cement)CathodeElectrolyteChemistryMetallurgyElectrode

Abstract

fetched live from OpenAlex

Electrochemical reactors can reduce the carbon intensity of cement production by using electricity to convert limestone (CaCO3) into Ca(OH)2, which can then be combined with silica (SiO2) at high temperatures to produce cement clinker. A key challenge with this method is the deposition of solid Ca(OH)2 at the reactor membrane leads to unacceptably low energy efficiencies. To address this challenge, we connected the electrochemical reactor (“cement electrolyser”) to a distinctive chemical reactor (“calcium reactor”) so that Ca(OH)2 could form there instead, and not within the electrochemical reactor. In this tandem system, the cement electrolyser generated H+ and OH– in the respective chemical and cathode compartments. The H+ then reacted with CaCO3 to form Ca2+ ions, which were diverted into the calcium reactor to react with the OH– to form Ca(OH)2. We fabricated a composite membrane to selectively block the transport of Ca2+ into the cathode compartment. Charge balance in the cement reactor was enabled with monovalent ions (e.g., K+) as the positive charge carrier. This orthgonalized ion management was validated by operando imaging. The tandem reactor enabled the electrolysis process to operate for 50 hours at 100 mA cm-2 without any voltage increase, which represents a meaningful step forward for cement clinker precursor production.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.632
Threshold uncertainty score0.936

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.241
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it