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Record W4377833565 · doi:10.1039/d3cc01512b

Plasmonic nanomaterials for solar-driven photocatalysis

2023· review· en· W4377833565 on OpenAlexafffund
Qingzhe Zhang, Zhihong Zuo, Dongling Ma

Bibliographic record

VenueChemical Communications · 2023
Typereview
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsInstitut National de la Recherche Scientifique
FundersFonds de recherche du Québec – Nature et technologiesTaishan Scholar Project of Shandong ProvinceNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of ChinaCanada Research Chairs
KeywordsPhotocatalysisPlasmonNanomaterialsNanotechnologyMaterials sciencePlasmonic nanoparticlesChemistryOptoelectronicsCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

Plasmonic nanomaterials have spurred significant research interest in enhanced solar-driven photocatalysis due to their strong localized surface plasmon resonance (LSPR). As this rapid-developing research area has begun to raise and answer fundamental questions that determine the photocatalytic performance of plasmonic photocatalysts, it is an opportune time to evaluate the advancement and propose future trajectories. We first outline the fundamentals of LSPR, including its excitation, decay, and influencing factors. We then discuss three main enhancement mechanisms and their applicable scenarios for plasmonic photocatalysis. We then critically assess the recent works performed by our groups concerning plasmon-enhanced photocatalytic reactions. By introducing related works from other researchers, we demonstrate our contributions to the advancements of plasmonic photocatalysis. Finally, we discuss the current challenges and suggest future directions in three aspects: material development, mechanism exploration, and application extension. It is anticipated to delineate the state-of-the-art and direct future research in plasmon-enhanced value-added chemical transformations.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.964
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0040.002
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.155
GPT teacher head0.415
Teacher spread0.260 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designNot applicable
Domainnot available
GenreReview

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations28
Published2023
Admission routes2
Has abstractyes

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